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Ni supported on the CaO modified attapulgite as catalysts for hydrogen production from glycerol steam reforming
Feng, P.1; Huang, K.2; Xu, Q.1,2; Qi, W.3; Xin, S.4; Wei, T.1; Liao, L.1; Yan, Y.1
2020-03-18
发表期刊INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
ISSN0360-3199
卷号45期号:15页码:8223-8233
通讯作者Xu, Q.(xuqingli@ecust.edu.cn) ; Qi, W.(qiwei@ms.giec.ac.cn)
摘要The Ni catalyst supported on CaO-modified attapulgite (CaO-ATP) were synthesized by wet impregnation method at a constant Ni metal loading (10 wt%). The catalyst was tested by carrying out a glycerin steam reforming reaction under the following conditions: 400-800 degrees C, W/G is 3, GHSV is 1 h(-1). Ni-CaO-ATP exhibited the highest hydrogen yield (85.30%) and glycerol conversion (93.71%) at 600 degrees C. The catalysts were characterized by N-2 adsorption/desorption, BET, XRD, H-2-TPR, TG and SEM. The results show that ATP has good resistance to carbon deposition. As an attapulgite modifier of Ni-CaO-ATP, CaO promotes the dispersion of the active component nickel species, which would promote the water gas shift reaction, leading to the improving of hydrogen yield. In addition, the addition of Ca would further enhance the inhibition of carbon deposition and prolong the life of the Ni -CaO-ATP catalyst. (C) 2020 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
关键词Hydrogen Steam reforming Attapulgite Ni catalysts CaO
DOI10.1016/j.ijhydene.2020.01.013
关键词[WOS]RU-BASED CATALYSTS ; NI/ATTAPULGITE CATALYSTS ; BIODIESEL PRODUCTION ; BIO-OIL ; TEMPERATURE ; ETHANOL ; PRETREATMENT ; GENERATION ; ACID ; CO
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[21376084] ; Guangxi Key Laboratory of Bio-refinery[GXKLB19-03] ; Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development[Y909kn1001]
WOS研究方向Chemistry ; Electrochemistry ; Energy & Fuels
项目资助者National Natural Science Foundation of China ; Guangxi Key Laboratory of Bio-refinery ; Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development
WOS类目Chemistry, Physical ; Electrochemistry ; Energy & Fuels
WOS记录号WOS:000523643400019
出版者PERGAMON-ELSEVIER SCIENCE LTD
引用统计
被引频次:42[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/27050
专题中国科学院广州能源研究所
通讯作者Xu, Q.; Qi, W.
作者单位1.East China Univ Sci & Technol, Res Ctr Biomass Energy, Key Lab Coal Gasificat & Energy Chem Engn, Minist Educ, Shanghai, Peoples R China
2.Guangxi Acad Sci, Natl Engn Res Ctr Nonfood Biorefinery, Guangxi Key Lab Biorefinery, Nanning, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou, Peoples R China
4.Jianghan Univ, Hubei Key Lab Ind Fume & Dust Pollut Control, Wuhan, Peoples R China
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GB/T 7714
Feng, P.,Huang, K.,Xu, Q.,et al. Ni supported on the CaO modified attapulgite as catalysts for hydrogen production from glycerol steam reforming[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2020,45(15):8223-8233.
APA Feng, P..,Huang, K..,Xu, Q..,Qi, W..,Xin, S..,...&Yan, Y..(2020).Ni supported on the CaO modified attapulgite as catalysts for hydrogen production from glycerol steam reforming.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,45(15),8223-8233.
MLA Feng, P.,et al."Ni supported on the CaO modified attapulgite as catalysts for hydrogen production from glycerol steam reforming".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 45.15(2020):8223-8233.
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