Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
| Reactivity and deactivation mechanisms of toluene reforming over waste peat char-supported Fe/Ni/Ca catalyst | |
Wang, Shuxiao1,2,3,4; Shan, Rui1,2,3,4; Gu, Jing1,2,3,4; Zhang, Jun1,2,3,4; Zhang, Yuyuan5; Yuan, Haoran1,2,3,4 ; Chen, Yong1,2,3,4; Luo, Bo6
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| 2020-07-01 | |
| Source Publication | FUEL
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| ISSN | 0016-2361 |
| Volume | 271Pages:8 |
| Corresponding Author | Yuan, Haoran(yuanhr@ms.giec.ac.cn) |
| Abstract | The pyrolysis char from waste peat with impregnated metal (Fe/Ni/Ca) were investigated for catalytic reforming of toluene in a laboratory dual-stage reactor. The prepared catalysts were examined in microstructure and textural characterization to analyze catalytic performance and stability. The results indicated that under the optimized conditions, the toluene conversions are greater than 92.7% for three types of peat char-supported catalysts, and the maximum molar ratio of syngas (CO + H-2) can reach up to 94.7% using Ni/peat char catalyst. The promising results demonstrated that the H-2 and CO are favored for Fe/peat char and Ni/peat char catalysts while the H-2 and CH4 are favored for Ca/peat char catalyst. After 320 min of experiment, the mol% of syngas decreased by less than 30% for three types of peat char catalysts. Significantly, peat char (C-SiO2) as a carrier can enhance the performance of catalyst through interaction with the metal, and it can be used as an adsorption carrier to absorb unreacted toluene. Such peat char-supported catalysts are thus promising for tar conversion and useful syngas production. |
| Keyword | Tar conversion Pyrolysis Catalyst Char Steam reforming Waste peat |
| DOI | 10.1016/j.fuel.2020.117517 |
| WOS Keyword | MUNICIPAL SOLID-WASTE ; TAR MODEL COMPOUNDS ; MICROWAVE PYROLYSIS ; SYNGAS PRODUCTION ; MOSO BAMBOO ; BOTTOM ASH ; RICE HUSK ; BIO-OIL ; CRACKING ; TRANSESTERIFICATION |
| Indexed By | SCI |
| Language | 英语 |
| Funding Project | National Key R&D Program of China[2018YFC1901200] ; National Natural Science Foundation of China[51906248] ; National Natural Science Foundation of China[51608507] ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory[GML2019ZD0101] ; Science and Technology Planning Project of Guangdong Province[2017B040404009] ; Guangdong Province Key Laboratory of Efficient and Clean Energy Utilization[2019ECEU02] |
| WOS Research Area | Energy & Fuels ; Engineering |
| Funding Organization | National Key R&D Program of China ; National Natural Science Foundation of China ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory ; Science and Technology Planning Project of Guangdong Province ; Guangdong Province Key Laboratory of Efficient and Clean Energy Utilization |
| WOS Subject | Energy & Fuels ; Engineering, Chemical |
| WOS ID | WOS:000522876500078 |
| Publisher | ELSEVIER SCI LTD |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.giec.ac.cn/handle/344007/26972 |
| Collection | 中国科学院广州能源研究所 |
| Corresponding Author | Yuan, Haoran |
| Affiliation | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, 2 Nengyuan Rd, Guangzhou 510640, Guangdong, Peoples R China 2.Southern Marine Sci & Engn Guangdong Lab, Guangzhou 511458, Peoples R China 3.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 4.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 5.Foshan Univ, Coll Mat Sci & Energy Engn, Foshan 528000, Peoples R China 6.Chongqing Environm & Sanitat Grp Co LTD, Chongqing, Peoples R China |
| First Author Affilication | GuangZhou Institute of Energy Conversion,Chinese Academy of Sciences |
| Recommended Citation GB/T 7714 | Wang, Shuxiao,Shan, Rui,Gu, Jing,et al. Reactivity and deactivation mechanisms of toluene reforming over waste peat char-supported Fe/Ni/Ca catalyst[J]. FUEL,2020,271:8. |
| APA | Wang, Shuxiao.,Shan, Rui.,Gu, Jing.,Zhang, Jun.,Zhang, Yuyuan.,...&Luo, Bo.(2020).Reactivity and deactivation mechanisms of toluene reforming over waste peat char-supported Fe/Ni/Ca catalyst.FUEL,271,8. |
| MLA | Wang, Shuxiao,et al."Reactivity and deactivation mechanisms of toluene reforming over waste peat char-supported Fe/Ni/Ca catalyst".FUEL 271(2020):8. |
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