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A facile method to improve the stability and efficiency of CsPbI2Br perovskite solar cells prepared at low temperature
Liu, Hongsha1,2; Xiao, Xiudi2; Bi, Zhuoneng2; Wang, Jixi2; Liu, Yangbiao2; Zhu, Yanqing2; Xu, Xueqing2; Xu, Gang1,2
2020
发表期刊SOLAR ENERGY
ISSN0038-092X
卷号195页码:544-551
通讯作者Xiao, Xiudi(xiaoxd@ms.giec.ac.cn) ; Xu, Gang(xugang@ms.giec.ac.cn)
摘要CsPbI2Br has become the focus of researchers in recent years due to its excellent thermal stability compared to the organic-inorganic hybrid perovskites. However, it requires high temperature to form cubic phase, and it is difficult to maintain the cubic phase in the high humidity ambient. By adding 30 mu L levulinic acid (LA) to the CsPbI2Br precursor solution, cubic phase CsPbI2Br can be obtained by spin-coating three minutes (TMS) at room temperature (RT) instead of high temperature. Based on the TMS, highly quality cubic phase CsPbI2Br film can be obtained at 80 degrees C annealing temperature, the stability of cubic phase CsPbI2Br can be significantly improved by adding LA in the CsPbI2Br precursor solution. Based on this, CsPbI2Br cells without LA achieve 11.68% power conversion efficiency (PCE) at low temperature of 80 degrees C and the corresponding stabilized power output is 10.31%. Furthermore, 10 mu L LA addition CsPbI2Br cells keep its 50% PCE after 10 days under 35%RH and RT. This has found a new way to improve the stability of inorganic perovskite solar cells, and increasing its potential in flexible solar cells.
关键词CsPbI2Br Levulinic acid Spin-coating three minutes Room temperature 80 degrees C
DOI10.1016/j.solener.2019.11.047
关键词[WOS]HALIDE PEROVSKITES ; ALPHA-CSPBI3 ; INTERFACE ; GAP
收录类别SCI
语种英语
资助项目National Key R&D Program of China[2018YFD0700200] ; Youth Innovation Promotion Association CAS[2017400] ; Special Plan of Guangdong Province[2015TQ01N714] ; Natural Science Foundation of Guangdong Province[2018A0303130146] ; Project of Science and Technology of Guangzhou[201904010171]
WOS研究方向Energy & Fuels
项目资助者National Key R&D Program of China ; Youth Innovation Promotion Association CAS ; Special Plan of Guangdong Province ; Natural Science Foundation of Guangdong Province ; Project of Science and Technology of Guangzhou
WOS类目Energy & Fuels
WOS记录号WOS:000509632000051
出版者PERGAMON-ELSEVIER SCIENCE LTD
引用统计
被引频次:7[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/26377
专题中国科学院广州能源研究所
通讯作者Xiao, Xiudi; Xu, Gang
作者单位1.Univ Sci & Technol China, Hefei 230031, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
第一作者单位中国科学院广州能源研究所
推荐引用方式
GB/T 7714
Liu, Hongsha,Xiao, Xiudi,Bi, Zhuoneng,et al. A facile method to improve the stability and efficiency of CsPbI2Br perovskite solar cells prepared at low temperature[J]. SOLAR ENERGY,2020,195:544-551.
APA Liu, Hongsha.,Xiao, Xiudi.,Bi, Zhuoneng.,Wang, Jixi.,Liu, Yangbiao.,...&Xu, Gang.(2020).A facile method to improve the stability and efficiency of CsPbI2Br perovskite solar cells prepared at low temperature.SOLAR ENERGY,195,544-551.
MLA Liu, Hongsha,et al."A facile method to improve the stability and efficiency of CsPbI2Br perovskite solar cells prepared at low temperature".SOLAR ENERGY 195(2020):544-551.
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