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Gasification performance of biowaste-derived hydrochar: The properties of products and the conversion processes
Zhuang, Xiuzheng1,4; Song, Yanpei1,4; Zhan, Hao2,3; Yin, Xiuli1; Wu, Chuangzhi1,4
2020-01-15
发表期刊FUEL
ISSN0016-2361
卷号260页码:11
通讯作者Yin, Xiuli(xlyin@ms.giec.ac.cn)
摘要Hydrothermal carbonization (HTC) coupled with gasification is recognized as an effective approach to produce hydrogen-rich syngas from biowastes, but only a few studies concerning the gasification capacity of various biowaste-derived hydrochars have been published yet. In this work, three types of biowaste (i.e., lignocellulosic, non-lignocellulosic and ash-rich types) were selected for the HTC experiments, and the subsequent gasification of hydrochars was carried out to investigate its thermogravimetric curves and the properties of products (i.e., syngas, tar and biochar). The results found that HTC improves the gasification efficiency in terms of the syngas quality and the conversion degree of sample. The concentrations of H-2 and CH4 in syngas were increased, while the gasified tar from hydrochars was concurrently reduced to half of its original value from biowastes under similar conditions. Furthermore, as HTC progressed, the gasification period and dynamic kinetics of samples exhibited slightly different, but the variation in the conversion process of gasification was similar; biowaste diversity in components is the reason for the former, while the developed aromatic structures in hydrochars is the explanation for the latter. These findings can not only provide a comprehensive knowledge on the gasification conversion of hydrochar, but also give a referential observation for designing, optimizing as well as scaling up the thermochemical conversion of industrial biowastes.
关键词Industrial biowastes Hydrothermal carbonization Gasification behaviors Reactivity
DOI10.1016/j.fuel.2019.116320
关键词[WOS]HYDROTHERMAL CARBONIZATION ; SEWAGE-SLUDGE ; STEAM GASIFICATION ; COMBUSTION BEHAVIOR ; INDUSTRIAL BIOWASTES ; SOLID-FUEL ; BIOMASS ; PYROLYSIS ; EVOLUTION ; KINETICS
收录类别SCI
语种英语
资助项目National Key Research and Development Program of China[2016YFE0203300] ; National Natural Science Foundation of China[51661145022] ; Science and Technology Program of Guangdong Province[2018A050506068] ; China Scholarship Council[201804910597]
WOS研究方向Energy & Fuels ; Engineering
项目资助者National Key Research and Development Program of China ; National Natural Science Foundation of China ; Science and Technology Program of Guangdong Province ; China Scholarship Council
WOS类目Energy & Fuels ; Engineering, Chemical
WOS记录号WOS:000491885400041
出版者ELSEVIER SCI LTD
引用统计
被引频次:37[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/26261
专题中国科学院广州能源研究所
通讯作者Yin, Xiuli
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Geochem, Guangdong Key Lab Environm Protect & Resources Ut, Guangzhou 510640, Guangdong, Peoples R China
4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
第一作者单位中国科学院广州能源研究所
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GB/T 7714
Zhuang, Xiuzheng,Song, Yanpei,Zhan, Hao,et al. Gasification performance of biowaste-derived hydrochar: The properties of products and the conversion processes[J]. FUEL,2020,260:11.
APA Zhuang, Xiuzheng,Song, Yanpei,Zhan, Hao,Yin, Xiuli,&Wu, Chuangzhi.(2020).Gasification performance of biowaste-derived hydrochar: The properties of products and the conversion processes.FUEL,260,11.
MLA Zhuang, Xiuzheng,et al."Gasification performance of biowaste-derived hydrochar: The properties of products and the conversion processes".FUEL 260(2020):11.
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