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Pd nanochains: Controlled synthesis by lysine and application in microbial fuel cells
Yang, Gaixiu1,2; Wang, Yufei1; Xu, Libang3; Li, Ying1; Li, Lianhua1; Sun, Yongming1; Yuan, Zhenhong1; Tang, Yawen2
2020
Source PublicationCHEMICAL ENGINEERING JOURNAL
ISSN1385-8947
Volume379Pages:8
Corresponding AuthorSun, Yongming(sunym@ms.giec.ac.cn) ; Tang, Yawen(tangyawen@njnu.edu.cn)
AbstractThree-dimensional networks composed of one-dimensional nanomaterials are widely used in electrocatalysis owing to their high charge transfer efficiencies. In this study, we report a hydrothermal lysine-assisted route for the synthesis of the Pd nanochain networks (Pd NCNs). In addition, we demonstrate the application of Pd NCNs in microbial fuel cells (MFCs), which represent a promising technology for wastewater treatment that also directly generates electrical energy. The Pd NCNs exhibit superior activity for the oxygen reduction reaction under neutral conditions because of their unique structure and down-shifted Pd d-band center, as compared with the commercial Pd black catalyst. The maximum power density generated in a membraneless single chamber MFC operating on wastewater with the as-prepared Pd NCNs as cathode catalysts is similar to 14.10 W m(-3) or 563.99 mW m(-2), which remains stable for over 100 days, clearly demonstrating the potential application of Pd NCNs in MFCs.
KeywordPd nanochains Oxygen reduction reaction Cathode catalysts Microbial fuel cell Wastewater treatment
DOI10.1016/j.cej.2019.122230
WOS KeywordOXYGEN REDUCTION REACTION ; ENHANCED ELECTROCATALYTIC PERFORMANCE ; WASTE-WATER TREATMENT ; ONE-POT SYNTHESIS ; ASSISTED SYNTHESIS ; POWER-GENERATION ; FACILE SYNTHESIS ; NETWORKS ; NANOPARTICLES ; CATALYST
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51806224] ; Natural Science Foundation of Guangdong Province[2017A 030310280] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDA21050400]
WOS Research AreaEngineering
Funding OrganizationNational Natural Science Foundation of China ; Natural Science Foundation of Guangdong Province ; Strategic Priority Research Program of the Chinese Academy of Sciences
WOS SubjectEngineering, Environmental ; Engineering, Chemical
WOS IDWOS:000494799900013
PublisherELSEVIER SCIENCE SA
Citation statistics
Cited Times:24[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/26206
Collection中国科学院广州能源研究所
Corresponding AuthorSun, Yongming; Tang, Yawen
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China
2.Nanjing Normal Univ, Jiangsu Collaborat Innovat Ctr Biomed Funct Mat, Sch Chem & Mat Sci, Jiangsu Key Lab New Power Batteries, Nanjing 210023, Jiangsu, Peoples R China
3.Nanjing Tech Univ, Coll Overseas Educ, Nanjing 211816, Jiangsu, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Yang, Gaixiu,Wang, Yufei,Xu, Libang,et al. Pd nanochains: Controlled synthesis by lysine and application in microbial fuel cells[J]. CHEMICAL ENGINEERING JOURNAL,2020,379:8.
APA Yang, Gaixiu.,Wang, Yufei.,Xu, Libang.,Li, Ying.,Li, Lianhua.,...&Tang, Yawen.(2020).Pd nanochains: Controlled synthesis by lysine and application in microbial fuel cells.CHEMICAL ENGINEERING JOURNAL,379,8.
MLA Yang, Gaixiu,et al."Pd nanochains: Controlled synthesis by lysine and application in microbial fuel cells".CHEMICAL ENGINEERING JOURNAL 379(2020):8.
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