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Solid base pretreatment to improve the accessibility of lignocellulosic molecules for biomass recovery
Tan, Xuesong1,2; Yu, Qiang1,2; Zhao, Yue1,2; Zhuang, Xinshu1,2; Wang, Qiong1,2; Qi, Wei1,2; Zhang, Yu1,2; Yuan, Zhenhong1,2; Wang, Zhongming1,2; Qin, Yanlin2,3; Guo, Ying1,2
2019-10-01
Source PublicationCELLULOSE
ISSN0969-0239
Volume26Issue:15Pages:8453-8464
Corresponding AuthorYu, Qiang(yuqiang@ms.giec.ac.cn) ; Zhuang, Xinshu(zhuangxs@ms.giec.ac.cn) ; Guo, Ying(guoying@ms.giec.ac.cn)
AbstractPretreatment with solid base catalysts addressed the challenge of recalcitrance of the lignocellulosic cell wall and provided insight into an economical and environmentally friendly biorefinery technology. Several solid base catalysts were prepared, to establish a reliable assessment of the factors governing their catalytic behaviors. The activity of solid base catalysts, allowing the more accessible lignocellulosic molecules to be depolymerized by enzymes, were evaluated by investigating the properties of the catalysts, the pretreated feedstock, and the residues, after 72 h of enzymatic hydrolysis. A statistical design (CCD) approach was applied to define the factors for the maximum saccharification and an efficient activity recovery. In the case of hybrid pennisetum, an optimized yield of 92% and a retention of 98% activity after 4 cycles were obtained. One of the mechanisms of the solid base catalysts during recalcitrance removal reactions, considering their structures and chemical compositions, was to enhance the accessibility of the cellulosic molecules.
KeywordLignocellulosic biomass Solid base Delignification Alkalinity Enzymatic hydrolysis
DOI10.1007/s10570-019-02564-0
WOS KeywordLAYERED DOUBLE HYDROXIDES ; MAGNESIUM-OXIDE ; ACTIVE OXYGEN ; CATALYSTS ; TECHNOLOGIES ; FUNDAMENTALS ; PYROLYSIS ; CHEMISTRY ; COOKING ; ALKALI
Indexed BySCI
Language英语
Funding ProjectNational Key R&D Program of China[2018YFB1501402] ; National Natural Science Foundation of China[51476179] ; National Natural Science Foundation of China[21476233] ; National Natural Science Foundation of China[51606203] ; Young Top-notch Talent of Guangdong Province, China[2016TQ03N647] ; Pearl River S&T Nova Program of Guangzhou, China[201610010110] ; Key Project of the Natural Science Foundation of Guangdong Province[2015A030311022] ; Open Fund of Guangdong Key Laboratory for Innovative Development and Utilization of Forest Plant Germplasm, South China Agricultural University ; Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development[Y807s71001] ; Youth Innovation Promotion Association, CAS[2015289]
WOS Research AreaMaterials Science ; Polymer Science
Funding OrganizationNational Key R&D Program of China ; National Natural Science Foundation of China ; Young Top-notch Talent of Guangdong Province, China ; Pearl River S&T Nova Program of Guangzhou, China ; Key Project of the Natural Science Foundation of Guangdong Province ; Open Fund of Guangdong Key Laboratory for Innovative Development and Utilization of Forest Plant Germplasm, South China Agricultural University ; Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development ; Youth Innovation Promotion Association, CAS
WOS SubjectMaterials Science, Paper & Wood ; Materials Science, Textiles ; Polymer Science
WOS IDWOS:000489757400019
PublisherSPRINGER
Citation statistics
Cited Times:3[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/25816
Collection中国科学院广州能源研究所
Corresponding AuthorYu, Qiang; Zhuang, Xinshu; Guo, Ying
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
2.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China
3.Guangdong Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Tan, Xuesong,Yu, Qiang,Zhao, Yue,et al. Solid base pretreatment to improve the accessibility of lignocellulosic molecules for biomass recovery[J]. CELLULOSE,2019,26(15):8453-8464.
APA Tan, Xuesong.,Yu, Qiang.,Zhao, Yue.,Zhuang, Xinshu.,Wang, Qiong.,...&Guo, Ying.(2019).Solid base pretreatment to improve the accessibility of lignocellulosic molecules for biomass recovery.CELLULOSE,26(15),8453-8464.
MLA Tan, Xuesong,et al."Solid base pretreatment to improve the accessibility of lignocellulosic molecules for biomass recovery".CELLULOSE 26.15(2019):8453-8464.
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