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Sedimentary geochemical proxies for methane seepage at Site C14 in the Qiongdongnan Basin in the northern South China Sea
Sun, Tiantian1,2; Wu, Daidai2,3; Yang, Fei2; Liu, Lihua2; Chen, Xuegang1; Ye, Ying1
2019-07-01
Source PublicationACTA OCEANOLOGICA SINICA
ISSN0253-505X
Volume38Issue:7Pages:84-95
Corresponding AuthorWu, Daidai(wudd@ms.giec.ac.cn)
AbstractRecent studies have shown that specific geochemical characteristics of sediments can be used to reconstruct past methane seepage events. In this work, the correlation between the Sr/Ca and Mg/Ca ratios of sediment samples is analyzed and the sulfate concentration profile in Site C14 from cold-seep sediments in the Qiongdongnan Basin in northern South China Sea is obtained. The results confirmed that, sulfate at 0-247 cm below sea floor (Unit I) is mainly consumed by organic matter sulfate reduction (OSR), while sulfate at 247-655 cm (Unit II) is consumed by both the OSR and the anaerobic oxidation of methane (AOM). In addition, the bottom sediment layer is affected by weak methane seepage. The Mo and U enrichment factors also exhibit similar trends in their respective depth profiles. The responses of trace elements, including Co/Al, Ni/Al, Cr/Al and Zn/Al ratios to methane seepage allowed the study of depositional conditions and methane seepage events. Based on the results, it is speculated that the depositional conditions of Unit II changed with depth from moderate conditions of sulfidic and oxic conditions to locally anoxic conditions, and finally to suboxic conditions due to methane fluid leakage. The stable isotope values of chromium-reducible sulfide produced by AOM and those of sulfide formed by OSR in the early diagenetic environment suffered serious depletion of S-34. This was probably due to weak methane leakage, which caused the slower upward diffusion and the effect of early diagenesis on the samples. It is necessary to consider the effects of depositional environments and diagenesis on these geochemical parameters.
KeywordQiongdongnan Basin trace elements stable isotope values anaerobic oxidation of methane methane activity
DOI10.1007/s13131-019-1460-6
WOS KeywordSOUTHWESTERN XISHA UPLIFT ; GAS HYDRATE ; PORE-WATER ; COLD SEEP ; AUTHIGENIC CARBONATES ; SHALLOW SEDIMENTS ; CONTINENTAL-SLOPE ; POCKMARK FIELD ; FLUID SOURCES ; MG/CA RATIOS
Indexed BySCI
Language英语
Funding ProjectProgram of Institution of South China Sea Ecology and Environmental Engineering, Chinese Academy of Sciences[ISEE2018YB03] ; Special Project for Marine Economy Development of Guangdong Province[GDME-2018D002] ; Evaluation and Detection Technology Laboratory for Marine Mineral Resources, Qingdao National Laboratory for Marine Science and Technology[KC201703] ; Youth Innovation Promotion Association CAS[201432]
WOS Research AreaOceanography
Funding OrganizationProgram of Institution of South China Sea Ecology and Environmental Engineering, Chinese Academy of Sciences ; Special Project for Marine Economy Development of Guangdong Province ; Evaluation and Detection Technology Laboratory for Marine Mineral Resources, Qingdao National Laboratory for Marine Science and Technology ; Youth Innovation Promotion Association CAS
WOS SubjectOceanography
WOS IDWOS:000476480800009
PublisherSPRINGER
Citation statistics
Cited Times:4[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/25457
Collection中国科学院广州能源研究所
Corresponding AuthorWu, Daidai
Affiliation1.Zhejiang Univ, Ocean Coll, Zhoushan 316021, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
3.Pilot Natl Lab Marine Sci & Technol Qingdao, Evaluat & Detect Technol Lab Marine Mineral Resou, Qingdao 266071, Shandong, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Sun, Tiantian,Wu, Daidai,Yang, Fei,et al. Sedimentary geochemical proxies for methane seepage at Site C14 in the Qiongdongnan Basin in the northern South China Sea[J]. ACTA OCEANOLOGICA SINICA,2019,38(7):84-95.
APA Sun, Tiantian,Wu, Daidai,Yang, Fei,Liu, Lihua,Chen, Xuegang,&Ye, Ying.(2019).Sedimentary geochemical proxies for methane seepage at Site C14 in the Qiongdongnan Basin in the northern South China Sea.ACTA OCEANOLOGICA SINICA,38(7),84-95.
MLA Sun, Tiantian,et al."Sedimentary geochemical proxies for methane seepage at Site C14 in the Qiongdongnan Basin in the northern South China Sea".ACTA OCEANOLOGICA SINICA 38.7(2019):84-95.
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