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Insights into induction time and agglomeration of methane hydrate formation in diesel oil dominated dispersed systems
Chen, Jun1,2; Chen, Guang-Jin3; Yuan, Qing4; Deng, Bin1; Tao, Li-Ming1; Li, Chuan-Hua1; Xiao, Sheng-Xiong1; Jiang, Jian-Hong1; Li, Xu1; Li, Jia-Yuan1
2019-03-01
发表期刊ENERGY
ISSN0360-5442
卷号170页码:604-610
通讯作者Chen, Jun(chenjun4174@126.com)
摘要Induction time and agglomeration of methane hydrate formation in dispersed systems play an important role in exploitation of natural gas hydrate, prevention of gas hydrate plug, and application of hydrate based technologies. In this work, an autoclave with particle video microscope (PVM) probe was used to detect induction time of methane hydrate formation as a function of the water cut, dosage of sorbitan monolaurate (Span 20), and subcooling. Forty-one experiments and thirty-six experiments of induction time have been conducted for methane hydrate formation at constant pressure and at nonconstant pressure, respectively. The results showed subcooling was the major factor that affects induction time during methane hydrate formation process. Subcooling of 4 K can be seen as an inflection point because the average methane hydrate formation time was less than 200 min when the subcooling was greater than 4 K, while methane hydrate formation time exhibited more stochastic when the subcooling was less than 4 K. The results also suggested that there exists a transformation range of subcooling (TRS) during methane hydrate formation process. The agglomerated mechanism of methane gas hydrate may be changed when the subcooling is greater than TRS, and subcooling of 4 K is included in the TRS. (C) 2018 Elsevier Ltd. All rights reserved.
关键词Hydrate Dispersed system Induction time Morphology Agglomeration Mechanism
DOI10.1016/j.energy.2018.12.138
关键词[WOS]NATURAL-GAS HYDRATE ; FLOW CHARACTERISTICS ; ANTI-AGGLOMERANTS ; PLUS WATER ; DISSOCIATION ; CYCLOPENTANE ; SLURRY ; SURFACTANT ; INHIBITORS ; MORPHOLOGY
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[21506065] ; Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion[Y707ke1001] ; Education Department of Hunan Province[16A197] ; Education Department of Hunan Province[17A199] ; Hunan Provincial Natural Science Foundation of China[2017JJ2240]
WOS研究方向Thermodynamics ; Energy & Fuels
项目资助者National Natural Science Foundation of China ; Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion ; Education Department of Hunan Province ; Hunan Provincial Natural Science Foundation of China
WOS类目Thermodynamics ; Energy & Fuels
WOS记录号WOS:000460845700052
出版者PERGAMON-ELSEVIER SCIENCE LTD
引用统计
被引频次:29[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/24777
专题中国科学院广州能源研究所
通讯作者Chen, Jun
作者单位1.Xiangnan Univ, Dept Chem & Life Sci, Hunan Prov Key Lab Xiangnan Rare Precious Met Cpd, Chenzhou 423000, Hunan, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
3.China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China
4.Liaocheng Univ, Sch Chem & Chem Engn, Liaocheng 252059, Peoples R China
第一作者单位中国科学院广州能源研究所
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Chen, Jun,Chen, Guang-Jin,Yuan, Qing,et al. Insights into induction time and agglomeration of methane hydrate formation in diesel oil dominated dispersed systems[J]. ENERGY,2019,170:604-610.
APA Chen, Jun.,Chen, Guang-Jin.,Yuan, Qing.,Deng, Bin.,Tao, Li-Ming.,...&Li, Jia-Yuan.(2019).Insights into induction time and agglomeration of methane hydrate formation in diesel oil dominated dispersed systems.ENERGY,170,604-610.
MLA Chen, Jun,et al."Insights into induction time and agglomeration of methane hydrate formation in diesel oil dominated dispersed systems".ENERGY 170(2019):604-610.
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