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A novel deep eutectic solvent from lignin-derived acids for improving the enzymatic digestibility of herbal residues from cellulose
Chen, Long1,3; Yu, Qiang1,2; Wang, Qiong1; Wang, Wen1; Qi, Wei1; Zhuang, Xinshu1; Wang, Zhongming1; Yuan, Zhenhong1
2019-02-01
Source PublicationCELLULOSE
ISSN0969-0239
Volume26Issue:3Pages:1947-1959
Corresponding AuthorYu, Qiang(yuqiang@ms.giec.ac.cn)
AbstractA novel lignin-derived deep eutectic solvent (DES) was synthesized from choline chloride (ChCl) and p-coumaric acid (PCA). The results showed that after pretreatment with lignin-derived DES, the dense cellulose-hemicellulose-lignin structure of herb residues of Cortex albiziae (HRCA) was effectively broken down and this facilitated subsequent enzymatic hydrolysis. The optimum pretreatment conditions were ChCl/PCA molar ratio of 1:1, 160 degrees C-5h, and a solid-liquid ratio of 1:10. Compared with untreated HRCA, 72-h enzymatic digestibility increased from 48.08 to 84.62%. When a ChCl-PCA-water pretreatment was used, the 72-h digestibility level of the residue reached 99.36%. Moreover, the recycling and reusability of this novel DES were evaluated. The results showed that synthesis and utilization of green, environment-friendly and recyclable lignin-derived DES can offer a new way of utilizing lignin which has considerable potential in the refining of biomass. [GRAPHICS] .
KeywordDeep eutectic solvents Enzymatic hydrolysis Lignin Pretreatment Structure changes
DOI10.1007/s10570-018-2190-8
WOS KeywordINORGANIC SALT PRETREATMENT ; LIGNOCELLULOSIC BIOMASS ; CHOLINE CHLORIDE ; RICE STRAW ; HYDROLYSIS ; TRANSFORMATION ; GASIFICATION ; TEMPERATURE
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51876206] ; National Natural Science Foundation of China[51506207] ; National Natural Science Foundation of China[21476233] ; Natural Science Foundation of Guangdong Province[2018A030313012] ; Young Top-Notch Talent of Guangdong Province, China[2016TQ03N647] ; Pearl River S&T Nova Program of Guangzhou, China[201610010110] ; DNL Cooperation Fund, CAS[DNL180305] ; Youth Innovation Promotion Association, CAS[2015289]
WOS Research AreaMaterials Science ; Polymer Science
Funding OrganizationNational Natural Science Foundation of China ; Natural Science Foundation of Guangdong Province ; Young Top-Notch Talent of Guangdong Province, China ; Pearl River S&T Nova Program of Guangzhou, China ; DNL Cooperation Fund, CAS ; Youth Innovation Promotion Association, CAS
WOS SubjectMaterials Science, Paper & Wood ; Materials Science, Textiles ; Polymer Science
WOS IDWOS:000460617900037
PublisherSPRINGER
Citation statistics
Cited Times:52[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/24665
Collection中国科学院广州能源研究所
Corresponding AuthorYu, Qiang
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China
2.Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100039, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Chen, Long,Yu, Qiang,Wang, Qiong,et al. A novel deep eutectic solvent from lignin-derived acids for improving the enzymatic digestibility of herbal residues from cellulose[J]. CELLULOSE,2019,26(3):1947-1959.
APA Chen, Long.,Yu, Qiang.,Wang, Qiong.,Wang, Wen.,Qi, Wei.,...&Yuan, Zhenhong.(2019).A novel deep eutectic solvent from lignin-derived acids for improving the enzymatic digestibility of herbal residues from cellulose.CELLULOSE,26(3),1947-1959.
MLA Chen, Long,et al."A novel deep eutectic solvent from lignin-derived acids for improving the enzymatic digestibility of herbal residues from cellulose".CELLULOSE 26.3(2019):1947-1959.
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