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Entrapment of Bi2O3 nanoparticles in TiO2 nanotubes for visible light-driven photocatalysis
Peng, Quanming1,3; Peng, Guiming2; Wu, Liangpeng1; Wang, Xiaoyang1,3; Yang, Xu1; Li, Xinjun1
2018-11-01
发表期刊RESEARCH ON CHEMICAL INTERMEDIATES
ISSN0922-6168
卷号44期号:11页码:6753-6763
通讯作者Li, Xinjun(lixj@ms.giec.ac.cn)
摘要In this study, we prepared nanoparticles of the visible light-responsive photocatalyst, Bi2O3 entrapped in anatase TiO2 nanotubes (Bi2O3-in-TNTs) via a vacuum-assisted precursor-filling process followed by annealing. Owing to the unique tubular electronic structure of TiO2 nanotubes, the interior of the nanotube is in an electron-deficient state, which was confirmed by XPS spectra and H-2-TPR. Electrochemical impedance studies showed that the Bi2O3-in-TNTs demonstrated a more efficient separation of photogenerated carriers than when Bi2O3 nanoparticles were deposited on the outer wall of TiO2 nanotubes (Bi2O3-out-TNTs). Due to the confinement effect of TiO2 nanotubes, which inhibits photogenerated carriers' recombination, the Bi2O3-in-TNTs exhibited a better photocatalytic performance for the photo-degradation of methyl orange under visible light compared to Bi2O3-out-TNTs.
关键词TiO2 nanotubes Bi2O3 Confinement effect Visible light Photocatalysis
DOI10.1007/s11164-018-3520-z
关键词[WOS]PERFORMANCE ; NANOCOMPOSITES ; COMPOSITE
收录类别SCI
语种英语
资助项目Science and Technology Program of Guangzhou, China[201803030019] ; Natural Science Foundation of Guangdong Province[2015A030313715] ; Natural Science Foundation of Jiangxi Province[20171BAB213010] ; Analytical & Testing Center, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, China
WOS研究方向Chemistry
项目资助者Science and Technology Program of Guangzhou, China ; Natural Science Foundation of Guangdong Province ; Natural Science Foundation of Jiangxi Province ; Analytical & Testing Center, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, China
WOS类目Chemistry, Multidisciplinary
WOS记录号WOS:000449307900020
出版者SPRINGER
引用统计
被引频次:15[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/24251
专题中国科学院广州能源研究所
通讯作者Li, Xinjun
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangdong Prov Key Lab New & Renewable Energy Res, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
2.Guangdong Univ Technol, Sch Mat & Energy, Guangzhou 510006, Guangdong, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
第一作者单位中国科学院广州能源研究所
推荐引用方式
GB/T 7714
Peng, Quanming,Peng, Guiming,Wu, Liangpeng,et al. Entrapment of Bi2O3 nanoparticles in TiO2 nanotubes for visible light-driven photocatalysis[J]. RESEARCH ON CHEMICAL INTERMEDIATES,2018,44(11):6753-6763.
APA Peng, Quanming,Peng, Guiming,Wu, Liangpeng,Wang, Xiaoyang,Yang, Xu,&Li, Xinjun.(2018).Entrapment of Bi2O3 nanoparticles in TiO2 nanotubes for visible light-driven photocatalysis.RESEARCH ON CHEMICAL INTERMEDIATES,44(11),6753-6763.
MLA Peng, Quanming,et al."Entrapment of Bi2O3 nanoparticles in TiO2 nanotubes for visible light-driven photocatalysis".RESEARCH ON CHEMICAL INTERMEDIATES 44.11(2018):6753-6763.
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