Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
| Hydrate-based acidic gases capture for clean methane with new synergic additives | |
Xia, Zhi-ming1,2; Li, Xiao-sen1,2 ; Chen, Zhao-yang1,2; Li, Gang1,2; Cai, Jing1,2,3; Wang, Yi1,2; Yan, Ke-feng1,2; Xu, Chun-gang1,2
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| 2017-12-01 | |
| Source Publication | APPLIED ENERGY
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| ISSN | 0306-2619 |
| Volume | 207Pages:584-593 |
| Corresponding Author | Li, Xiao-sen(lixs@ms.giec.ac.cn) |
| Abstract | The widespread need for carbon dioxide (CO2) and hydrogen sulfide (H2S) removal from potential. gaseous fuel processes associated with upgrading of natural gas, biogas and landfill gas has led to a continuing interest in developing acid gas capture technologies. This work experimentally investigated the hydrate-based acidic gases (CO2 and H2S) capture for clean methane (CH4) fuel from biogas or natural gas with new synergic additives, which comprised physical gas solvent (TMS) and traditional hydrate promoter (TBAB). The results show that, with the synergic additives, the equilibrium hydrate formation pressures were moderated by about 90% relative to pure water, the selectivity of CO2 over CH4 and the selectivity of H2S over CH4 could achieve 18.56 and 11.38, respectively. Compared with TBAB, the synergic additives could improve the hydrate formation rate and the gas storage capacity by 149% and 84%, respectively. Furthermore, the promotion effect could be enhanced when with the help of H2S. It has been shown that CO2 and H2S could be synchronously captured through the hydrate formation process. It will be of importance to the fundamental study of enhancing gas hydrate formation process, and of practical significance for the hydrate-based application industry. (C) 2017 Elsevier Ltd. All rights reserved. |
| Keyword | Acidic gas Biogas Natural gas Hydrate Separation Synergic additives |
| DOI | 10.1016/j.apenergy.2017.06.017 |
| WOS Keyword | PRE-COMBUSTION CAPTURE ; FIXED-BED REACTOR ; SEPARATION HBGS PROCESS ; CARBON-DIOXIDE CAPTURE ; FLUE-GAS ; CO2 SEPARATION ; LANDFILL GAS ; PHASE-EQUILIBRIUM ; AQUEOUS-SOLUTIONS ; CLATHRATE PROCESS |
| Indexed By | SCI |
| Language | 英语 |
| Funding Project | National Natural Science Foundation of China[21306194] ; National Natural Science Foundation of China[51576202] ; National Natural Science Foundation of China[51676196] ; National Natural Science Foundation of China[51376184] ; International Science & Technology Cooperation Program of China[2015DFA61790] ; Frontier Sciences Key Research Program of the Chinese Academy of Sciences[QYZDJ-SSW-JSC033] ; CAS Science and Technology Apparatus Development Program[YZ201619] ; CAS & CNPC Cooperation Program[2015A-4813] ; Pearl River S&T Nova Program of Guangzhou[201710010098] ; Pearl River S&T Nova Program of Guangzhou[201610010164] |
| WOS Research Area | Energy & Fuels ; Engineering |
| Funding Organization | National Natural Science Foundation of China ; International Science & Technology Cooperation Program of China ; Frontier Sciences Key Research Program of the Chinese Academy of Sciences ; CAS Science and Technology Apparatus Development Program ; CAS & CNPC Cooperation Program ; Pearl River S&T Nova Program of Guangzhou |
| WOS Subject | Energy & Fuels ; Engineering, Chemical |
| WOS ID | WOS:000417229300051 |
| Publisher | ELSEVIER SCI LTD |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.giec.ac.cn/handle/344007/22562 |
| Collection | 中国科学院广州能源研究所 |
| Corresponding Author | Li, Xiao-sen |
| Affiliation | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou, Guangdong, Peoples R China 2.Guangdong Key Lab New & Renewable Energy, Guangzhou, Guangdong, Peoples R China 3.Univ Chinese Acad Sci, Beijing, Peoples R China |
| First Author Affilication | GuangZhou Institute of Energy Conversion,Chinese Academy of Sciences |
| Recommended Citation GB/T 7714 | Xia, Zhi-ming,Li, Xiao-sen,Chen, Zhao-yang,et al. Hydrate-based acidic gases capture for clean methane with new synergic additives[J]. APPLIED ENERGY,2017,207:584-593. |
| APA | Xia, Zhi-ming.,Li, Xiao-sen.,Chen, Zhao-yang.,Li, Gang.,Cai, Jing.,...&Xu, Chun-gang.(2017).Hydrate-based acidic gases capture for clean methane with new synergic additives.APPLIED ENERGY,207,584-593. |
| MLA | Xia, Zhi-ming,et al."Hydrate-based acidic gases capture for clean methane with new synergic additives".APPLIED ENERGY 207(2017):584-593. |
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