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Furfural Hydrogenation over Amorphous Alloy Catalysts Prepared by Different Reducing Agents
Guo, Haijun1,2,3,4,5; Zhang, Hairong1,2,3,4; Tang, Weichao1,2,3,4; Wang, Can1,2,3,4; Huang, Chao1,2,3,4; Chen, Peili1,2,3; Chen, Xinde1,2,3,4; Ouyang, Xinping5
2017
发表期刊BIORESOURCES
ISSN1930-2126
卷号12期号:4页码:8755-8774
通讯作者Chen, Xinde(cxd_cxd@hotmail.com)
摘要The catalytic hydrogenation of furfural was studied over a series of Ni-B, Co-B, and Ni-Co-B amorphous alloy catalysts that were prepared by the chemical reduction method using KBH4 and NaBH4 as reducing agents. These catalysts were characterized by N-2 adsorption/desorption, XRD, XPS, FE-SEM, and TEM. The results showed that NaBH4 had a much stronger reduction ability to enhance the surface concentration of the metallic active sites for furfural hydrogenation and electron transfer capability, leading to much higher hydrogenation activity. In the Ni-Co-B amorphous alloy catalyst, the equilibrium between the isolated Ni-B/Co-B active sites and the combined Ni-Co-B active sites was important in regulating furfural conversion and products distribution.
关键词Furfural hydrogenation Ni-Co-B amorphous alloy Reducing agent Synergistic effect Electron transfer capability
DOI10.15376/biores.12.4.8755-8774
关键词[WOS]LIQUID-PHASE HYDROGENATION ; PORE-SIZE DISTRIBUTION ; NI-B ; CO-B ; SELECTIVE HYDROGENATION ; CHEMICAL-REDUCTION ; ALCOHOL ; CONVERSION ; BOROHYDRIDE ; HYDROLYSIS
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[21406229] ; Project of Jiangsu Province Science and Technology[BE2014101] ; Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development[Y709jh1001]
WOS研究方向Materials Science
项目资助者National Natural Science Foundation of China ; Project of Jiangsu Province Science and Technology ; Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development
WOS类目Materials Science, Paper & Wood
WOS记录号WOS:000422879900130
出版者NORTH CAROLINA STATE UNIV DEPT WOOD & PAPER SCI
引用统计
被引频次:10[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/16737
专题中国科学院广州能源研究所
通讯作者Chen, Xinde
作者单位1.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
2.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
4.Chinese Acad Sci, Guangzhou Inst Energy Convers, R&D Ctr Xuyi Attapulgite Appl Technol, Xuyi 211700, Peoples R China
5.South China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
第一作者单位中国科学院广州能源研究所
推荐引用方式
GB/T 7714
Guo, Haijun,Zhang, Hairong,Tang, Weichao,et al. Furfural Hydrogenation over Amorphous Alloy Catalysts Prepared by Different Reducing Agents[J]. BIORESOURCES,2017,12(4):8755-8774.
APA Guo, Haijun.,Zhang, Hairong.,Tang, Weichao.,Wang, Can.,Huang, Chao.,...&Ouyang, Xinping.(2017).Furfural Hydrogenation over Amorphous Alloy Catalysts Prepared by Different Reducing Agents.BIORESOURCES,12(4),8755-8774.
MLA Guo, Haijun,et al."Furfural Hydrogenation over Amorphous Alloy Catalysts Prepared by Different Reducing Agents".BIORESOURCES 12.4(2017):8755-8774.
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