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One-Pot Conversion of Carbohydrates into 5-(Hydroxymethyl)furfural using Heterogeneous Lewis-Acid and Bronsted-Acid Catalysts
Zhang, Tingwei1; Fan, Wei2; Li, Wenzhi1; Xu, Zhiping3; Xin, Haosheng4; Su, Mingxue3; Lu, Yijuan1; Ma, Longlong5
2017-05-01
发表期刊ENERGY TECHNOLOGY
卷号5期号:5页码:747-755
摘要Sn-beta zeolite and PTSA-POM, made from the copolymerization of p-toluenesulfonic acid (PTSA) and paraformaldehyde (POM), were used for the production of 5-(hydroxymethyl)-furfural (HMF) from glucose in an environmentally friendly solvent system including gamma-valerolactone (GVL) and H2O. The effects of reaction temperature, reaction time, solvent, and catalyst-to-reactant ratio on the production of HMF were investigated. The combination of the Bronsted acid and Lewis acid catalysts largely improved the catalytic system and resulted in the production of HMF in 60.1% yield at 140 degrees C in 30min. The presence of water in the solvent had a positive influence on the production of HMF from glucose. The combination of the two catalysts also improved the catalytic performance for the production of HMF from cellulose and corn stalk.
文章类型Article
关键词Carbohydrates Cellulose Corn Stalk Heterogeneous Catalysis Sustainable Chemistry
WOS标题词Science & Technology ; Technology
资助者National Key Technology R&D Program of China(2015BAD15B06) ; National Basic Research Program of China(2012CB215302) ; Science and Technological Fund of Anhui Province for Outstanding Youth(1508085J01) ; International Technology Cooperation Plan of Anhui(1503062030) ; National Key Technology R&D Program of China(2015BAD15B06) ; National Basic Research Program of China(2012CB215302) ; Science and Technological Fund of Anhui Province for Outstanding Youth(1508085J01) ; International Technology Cooperation Plan of Anhui(1503062030)
DOI10.1002/ente.201600492
研究领域[WOS]Energy & Fuels
关键词[WOS]BIOMASS ENERGY CONVERSATION ; GAMMA-VALEROLACTONE ; IONIC LIQUIDS ; SN-BETA ; GLUCOSE ISOMERIZATION ; EFFICIENT CONVERSION ; LEVULINIC ACID ; AQUEOUS-MEDIA ; ACTIVE-SITES ; CORN STALK
收录类别SCI
语种英语
资助者National Key Technology R&D Program of China(2015BAD15B06) ; National Basic Research Program of China(2012CB215302) ; Science and Technological Fund of Anhui Province for Outstanding Youth(1508085J01) ; International Technology Cooperation Plan of Anhui(1503062030) ; National Key Technology R&D Program of China(2015BAD15B06) ; National Basic Research Program of China(2012CB215302) ; Science and Technological Fund of Anhui Province for Outstanding Youth(1508085J01) ; International Technology Cooperation Plan of Anhui(1503062030)
WOS类目Energy & Fuels
WOS记录号WOS:000401237900013
引用统计
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/14126
专题中国科学院广州能源研究所
作者单位1.Univ Sci & Technol China, Dept Thermal Sci & Energy Engn, 96 Jinzhai Rd, Hefei 230026, Anhui, Peoples R China
2.Univ Massachusetts, Chem Engn Dept, Goessmann Lab 177B, 686 N Pleasant St, Amherst, MA 01003 USA
3.Univ Sci & Technol China, Dept Chem, 96 Jinzhai Rd, Anhua 230026, Anhui, Peoples R China
4.Anhui Jiangzhu Univ, Inst Mat & Chem Engn, Hefei 230022, Peoples R China
5.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
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GB/T 7714
Zhang, Tingwei,Fan, Wei,Li, Wenzhi,et al. One-Pot Conversion of Carbohydrates into 5-(Hydroxymethyl)furfural using Heterogeneous Lewis-Acid and Bronsted-Acid Catalysts[J]. ENERGY TECHNOLOGY,2017,5(5):747-755.
APA Zhang, Tingwei.,Fan, Wei.,Li, Wenzhi.,Xu, Zhiping.,Xin, Haosheng.,...&Ma, Longlong.(2017).One-Pot Conversion of Carbohydrates into 5-(Hydroxymethyl)furfural using Heterogeneous Lewis-Acid and Bronsted-Acid Catalysts.ENERGY TECHNOLOGY,5(5),747-755.
MLA Zhang, Tingwei,et al."One-Pot Conversion of Carbohydrates into 5-(Hydroxymethyl)furfural using Heterogeneous Lewis-Acid and Bronsted-Acid Catalysts".ENERGY TECHNOLOGY 5.5(2017):747-755.
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