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The effect of tetrabutylphosphonium bromide on the formation process of CO2 hydrates
Shi, Lingli1,2,3; Yi, Lizhi1,2,3; Shen, Xiaodong1,2,3,4; Wu, Wenzhi1,2,3,4; Liang, Deqing1,2,3
2017-03-01
发表期刊JOURNAL OF MOLECULAR LIQUIDS
卷号229页码:98-105
摘要Quaternary salts can form semiclathrate hydrates with vacant cages to capture gas molecules, such as CO2. To study the effect in the formation process of CO2 hydrates, the formation kinetics of tetrabutylphosphonium bromide (TBPB) + CO2 hydrate were investigated in this work. The study was conducted by employing an isobaric method with salt mass fraction and subcooling degree ranging from (0.10 to 0.60) and from (8 K to 10 K), respectively. The kinetic performance of TBPB was evaluated by the induction time, normalized gas consumption, and normalized gas consumption rate. The results showed that the induction time decreased with the increase of subcooling degree as well as the salt mass fraction. When salt mass fraction exceeded 0.20, the average induction times were particularly short and almost the same. In addition, the salt mass fraction had a great impact on the normalized gas consumption rather than the normalized gas consumption rate. (C)2016 Elsevier B.V. All rights reserved.
文章类型Article
关键词Tetrabutylphosphonium Bromide Co2 Capture And Storage Hydrate Formation Kinetics
WOS标题词Science & Technology ; Physical Sciences
资助者National Natural Science Foundation of China(51376182) ; Guangdong Natural Sciences of Foundation(2016A030310126) ; Key Laboratory of Gas Hydrate ; Guangzhou Institute of Energy Conversion ; Chinese Academy of Sciences(Y607jb1001) ; National Natural Science Foundation of China(51376182) ; Guangdong Natural Sciences of Foundation(2016A030310126) ; Key Laboratory of Gas Hydrate ; Guangzhou Institute of Energy Conversion ; Chinese Academy of Sciences(Y607jb1001)
DOI10.1016/j.molliq.2016.12.038
研究领域[WOS]Chemistry ; Physics
关键词[WOS]PLUS CARBON-DIOXIDE ; N-BUTYLAMMONIUM BROMIDE ; PHASE-EQUILIBRIUM DATA ; GUEST GAS ENCLATHRATION ; BUTYL AMMONIUM-CHLORIDE ; AQUEOUS-SOLUTION SYSTEMS ; SIMULATED FLUE-GAS ; SEMICLATHRATE HYDRATE ; CLATHRATE HYDRATE ; DISSOCIATION CONDITIONS
收录类别SCI
语种英语
资助者National Natural Science Foundation of China(51376182) ; Guangdong Natural Sciences of Foundation(2016A030310126) ; Key Laboratory of Gas Hydrate ; Guangzhou Institute of Energy Conversion ; Chinese Academy of Sciences(Y607jb1001) ; National Natural Science Foundation of China(51376182) ; Guangdong Natural Sciences of Foundation(2016A030310126) ; Key Laboratory of Gas Hydrate ; Guangzhou Institute of Energy Conversion ; Chinese Academy of Sciences(Y607jb1001)
WOS类目Chemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS记录号WOS:000395598800012
引用统计
被引频次:3[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/14099
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, CAS Key Lab Gas Hydrate, Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China
3.Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou 510640, Guangdong, Peoples R China
4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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Shi, Lingli,Yi, Lizhi,Shen, Xiaodong,et al. The effect of tetrabutylphosphonium bromide on the formation process of CO2 hydrates[J]. JOURNAL OF MOLECULAR LIQUIDS,2017,229:98-105.
APA Shi, Lingli,Yi, Lizhi,Shen, Xiaodong,Wu, Wenzhi,&Liang, Deqing.(2017).The effect of tetrabutylphosphonium bromide on the formation process of CO2 hydrates.JOURNAL OF MOLECULAR LIQUIDS,229,98-105.
MLA Shi, Lingli,et al."The effect of tetrabutylphosphonium bromide on the formation process of CO2 hydrates".JOURNAL OF MOLECULAR LIQUIDS 229(2017):98-105.
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