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Aqueous-Phase Hydrodeoxygenation of Biomass Sugar Alcohol into Renewable Alkanes over a Carbon-Supported Ruthenium with Phosphoric Acid Catalytic System
Weng, Yujing1,2; Wang, Tiejun1; Qiu, Songbai1; Wang, Chenguang1; Ma, Longlong1; Zhang, Qi1; Chen, Lungang1; Li, Yuping1; Sun, Fei1; Zhang, Qian1,2
2017-03-01
发表期刊CHEMCATCHEM
卷号9期号:5页码:774-781
摘要Recently, we demonstrated the catalytic conversion of biomass hydrolysate and real biomass into renewable alkanes over a Ru/C catalyst with aqueous phosphoric acid (Ru/C+H3PO4) and we obtained a high yield of C-5/C-6 alkanes. In this study, the mechanism of sorbitol hydrodeoxygenation (HDO) into alkanes over the Ru/C+H3PO4 catalytic system was investigated by using a trickle-bed reactor. A high HDO performance was detected with a large amount of long-chain alkanes in the products. Subsequently, pre- and postcharacterization studies (N-2 adsorption, XRD, X-ray photoelectron spectroscopy, TEM, NH3 temperature-programmed desorption, H-2 temperature-programmed reduction, FTIR spectroscopy) were performed on the relevant catalysts to study the change of the catalytic active sites. Moreover, mineral acid experiments were performed to study the influence of phosphoric acid on the HDO performance.
文章类型Article
关键词Alcohols Alkanes Biomass Ruthenium Supported Catalysts
WOS标题词Science & Technology ; Physical Sciences
DOI10.1002/cctc.201601470
研究领域[WOS]Chemistry
关键词[WOS]STABLE HETEROGENEOUS CATALYSTS ; TRANSFER HYDROGENATION ; RU/C CATALYST ; SORBITOL TRANSFORMATION ; LIGNOCELLULOSIC BIOMASS ; OXYGEN REDUCTION ; CONVERSION ; PHOSPHATE ; DEHYDRATION ; EFFICIENT
收录类别SCI
语种英语
项目资助者National Natural Science Foundation of China(51476176 ; key program of Chinese Academy of Sciences(KGZD-EW-304-2) ; Guangdong province special Talent support plan(511054728068) ; 51536009)
WOS类目Chemistry, Physical
WOS记录号WOS:000395799000009
引用统计
被引频次:13[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/14085
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangdong Prov Key Lab New & Renewable Energy Res, Key Lab Renewable Energy, Nengyuan Rd 2, Guangzhou 510640, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
第一作者单位中国科学院广州能源研究所
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Weng, Yujing,Wang, Tiejun,Qiu, Songbai,et al. Aqueous-Phase Hydrodeoxygenation of Biomass Sugar Alcohol into Renewable Alkanes over a Carbon-Supported Ruthenium with Phosphoric Acid Catalytic System[J]. CHEMCATCHEM,2017,9(5):774-781.
APA Weng, Yujing.,Wang, Tiejun.,Qiu, Songbai.,Wang, Chenguang.,Ma, Longlong.,...&Zhang, Qian.(2017).Aqueous-Phase Hydrodeoxygenation of Biomass Sugar Alcohol into Renewable Alkanes over a Carbon-Supported Ruthenium with Phosphoric Acid Catalytic System.CHEMCATCHEM,9(5),774-781.
MLA Weng, Yujing,et al."Aqueous-Phase Hydrodeoxygenation of Biomass Sugar Alcohol into Renewable Alkanes over a Carbon-Supported Ruthenium with Phosphoric Acid Catalytic System".CHEMCATCHEM 9.5(2017):774-781.
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