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Ni/La2O3-ZrO2 catalyst for hydrogen production from steam reforming of acetic acid as a model compound of bio-oil
Xue, Ya-ping1,2,3,4; Yan, Chang-feng1,2,3,4; Zhao, Xiao-yong1,2,3,4; Huang, Shi-lin1,2,3; Guo, Chang-qing1,2,3
2017-02-01
发表期刊KOREAN JOURNAL OF CHEMICAL ENGINEERING
卷号34期号:2页码:305-313
摘要Hydrogen production from steam reforming of acetic acid was investigated over Ni/La2O3-ZrO2 catalyst. A series of Ni/La2O3-ZrO2 catalysts were synthesized by sol-gel method coupled with wet impregnation, which was characterized by XRD, BET, TEM, EDS, TG, SEM and TPR. Catalytic activity of Ni/La2O3-ZrO2 was evaluated by steam reforming of acetic acid at the temperature range of 550-750 A degrees C. The tetragonal phase La0.1Zr0.9O1.95 is formed through the doping of La2O3 into the ZrO2 lattice and nickel species are highly dispersed on the support with high specific surface area. H-2 yield and CO2 yield of Ni/La2O3-ZrO2 catalyst with 15%wt Ni reaches 89.27% and 80.41% at 600 A degrees C, respectively, which is attributed to high BET surface area and sufficient Ni active sites in strong interaction with the support. 15%wt Ni supported on La2O3-ZrO2 catalyst maintains relatively stable catalytic activities for a period of 20 h.
文章类型Article
关键词Hydrogen Production Ni/la2o3-zro2 Catalyst Steam Reforming Bio-oil Acetic Acid
WOS标题词Science & Technology ; Physical Sciences ; Technology
资助者CAS Renewable Energy Key Lab. ; Natural Science Foundation of China(51576201) ; National Natural Science Foundation of Guangdong province(2015A030312007) ; Guangdong Science and Technology Project(2013B050800007) ; Guangzhou Science and Technology Project(2013J4500027) ; CAS Renewable Energy Key Lab. ; Natural Science Foundation of China(51576201) ; National Natural Science Foundation of Guangdong province(2015A030312007) ; Guangdong Science and Technology Project(2013B050800007) ; Guangzhou Science and Technology Project(2013J4500027)
DOI10.1007/s11814-016-0277-1
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]STABLE CATALYSTS ; BIOMASS ; ETHANOL ; DEPOSITION ; MECHANISM ; ZIRCONIA ; METHANE ; SIZE
收录类别SCI
语种英语
资助者CAS Renewable Energy Key Lab. ; Natural Science Foundation of China(51576201) ; National Natural Science Foundation of Guangdong province(2015A030312007) ; Guangdong Science and Technology Project(2013B050800007) ; Guangzhou Science and Technology Project(2013J4500027) ; CAS Renewable Energy Key Lab. ; Natural Science Foundation of China(51576201) ; National Natural Science Foundation of Guangdong province(2015A030312007) ; Guangdong Science and Technology Project(2013B050800007) ; Guangzhou Science and Technology Project(2013J4500027)
WOS类目Chemistry, Multidisciplinary ; Engineering, Chemical
WOS记录号WOS:000394228000004
引用统计
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/14051
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
3.Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Guangdong, Peoples R China
4.Univ Chinese Acad Sci, Beijing 100039, Peoples R China
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Xue, Ya-ping,Yan, Chang-feng,Zhao, Xiao-yong,et al. Ni/La2O3-ZrO2 catalyst for hydrogen production from steam reforming of acetic acid as a model compound of bio-oil[J]. KOREAN JOURNAL OF CHEMICAL ENGINEERING,2017,34(2):305-313.
APA Xue, Ya-ping,Yan, Chang-feng,Zhao, Xiao-yong,Huang, Shi-lin,&Guo, Chang-qing.(2017).Ni/La2O3-ZrO2 catalyst for hydrogen production from steam reforming of acetic acid as a model compound of bio-oil.KOREAN JOURNAL OF CHEMICAL ENGINEERING,34(2),305-313.
MLA Xue, Ya-ping,et al."Ni/La2O3-ZrO2 catalyst for hydrogen production from steam reforming of acetic acid as a model compound of bio-oil".KOREAN JOURNAL OF CHEMICAL ENGINEERING 34.2(2017):305-313.
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