Fast preparation of uniform large grain size perovskite thin film in air condition via spray deposition method for high efficient planar solar cells

doi:10.1016/j.solmat2016.12.032

GIEC OpenIR > 中国科学院广州能源研究所

	Fast preparation of uniform large grain size perovskite thin film in air condition via spray deposition method for high efficient planar solar cells
	Bi, Zhuoneng 1,2; Liang, Zhurong 1,2; Xu, Xueqing1,2 ; Chai, Zhisheng 1,2; Jin, Hu 1,2; Xu, Dehua 1,2; Li, Jingling 1,2; Li, Minghua 3; Xu, Gang1,2
	2017-04-01
发表期刊	SOLAR ENERGY MATERIALS AND SOLAR CELLS
卷号	162 页码:13-20
摘要	Spray deposition has been demonstrated to be a promising method to prepare perovskite thin film with many advantages, such as easy and processable under fully ambient condition, which is suitable for large-scale production. In this work, we reveal two typical spray deposition process of rapid and slow solvent evaporation. It is emphasized that the rapid solvent evaporation process is essential to avoid dendritic crystal and obtain dense perovskite thin film without pin-holes, which can be realized with a suitable substrate temperature. With optimized spray conditions including flow rate of precursor solution and carrier gas pressure, a dense and uniform perovskite layer with full surface coverage was immediately formed in similar to 5 s without any post-annealing process. The as-fabricated planar heterojunction solar cell achieved a power conversion efficiency (PCE) of 13.54% with 300 +/- 30 nm in thickness of perovskite layer. To the best of our knowledge, this result is the highest value for the CH3NH3PbI3 perovskite solar cells fabricated in air condition with high humidity up to 50%.
文章类型	Article
关键词	Ch3nh3pbi3 Perovskite Thin Film Spray Deposition Fast Preparation High Efficient Planar Solar Cells
WOS标题词	Science & Technology ; Technology ; Physical Sciences
DOI	10.1016/j.solmat2016.12.032
研究领域[WOS]	Energy & Fuels ; Materials Science ; Physics
关键词[WOS]	PERFORMANCE ; GROWTH ; CRYSTALLIZATION ; FABRICATION ; HYSTERESIS
收录类别	SCI
语种	英语
项目资助者	National Natural Science Foundation of China(21073193 ; Natural Science Foundation of Guangdong Province(2015A030310501) ; Project on the Collaborative Innovation and Environmental Construction Platform of Guangdong Province(2014A050503051) ; 21273241)
WOS类目	Energy & Fuels ; Materials Science, Multidisciplinary ; Physics, Applied
WOS记录号	WOS:000393720500003
引用统计	被引频次：52[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.giec.ac.cn/handle/344007/14048
专题	中国科学院广州能源研究所
作者单位	1.Chinese Acad Sci, Guangdong Key Lab New & Renewable Energy Res & De, Key Lab Renewable Energy, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Guangdong Mech & Elect Polytech, Guangzhou 510515, Guangdong, Peoples R China
推荐引用方式 GB/T 7714	Bi, Zhuoneng,Liang, Zhurong,Xu, Xueqing,et al. Fast preparation of uniform large grain size perovskite thin film in air condition via spray deposition method for high efficient planar solar cells[J]. SOLAR ENERGY MATERIALS AND SOLAR CELLS,2017,162:13-20.
APA	Bi, Zhuoneng.,Liang, Zhurong.,Xu, Xueqing.,Chai, Zhisheng.,Jin, Hu.,...&Xu, Gang.(2017).Fast preparation of uniform large grain size perovskite thin film in air condition via spray deposition method for high efficient planar solar cells.SOLAR ENERGY MATERIALS AND SOLAR CELLS,162,13-20.
MLA	Bi, Zhuoneng,et al."Fast preparation of uniform large grain size perovskite thin film in air condition via spray deposition method for high efficient planar solar cells".SOLAR ENERGY MATERIALS AND SOLAR CELLS 162(2017):13-20.