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Effect of Ru Particle Size on Hydrogenation/Decarbonylation of Propanoic Acid Over Supported Ru Catalysts in Aqueous Phase
Chen, Lungang; Li, Yuping; Zhang, Xinghua; Zhang, Qi; Wang, Tiejun; Ma, Longlong
2017
发表期刊CATALYSIS LETTERS
卷号147期号:1页码:29-38
摘要The aqueous-phase hydrogenation of propanoic acid was performed over the Ru/ZrO2 and Ru/Al2O3 catalysts with different Ru loading. Combined with multiple characterization techniques, such as H-2-TPR, XRD, CO-FTIR, and DRIFTS of propanoic acid, the effect of Ru loading on the decarbonylation/hydrogenation of propanoic acid was investigated. Although hydrogenation/decarbonylation of carboxylic acids were strongly affected by the nature of supports, the increase of metal loading can cause the larger Ru particles and more bare Ru metal sites, which can facilitate the C-C bond cleavage reaction derived from the decarbonylation of propanoyl species over Ru metal sites.
文章类型Article
关键词Ru Loading Carboxylic Acid Hydrogenation Decarbonylation C-c Cleavage
WOS标题词Science & Technology ; Physical Sciences
资助者National Natural Science Foundation of China(51306189) ; Science and Technology Program of Guangdong Province(2014A010106022) ; Comprehensive Strategic Cooperation Project of Guangdong Province ; Chinese Academy of Sciences(2012B090400042) ; China-EU SMEs Cooperation Fund for Energy Conservation Research Project(SQ2013ZOB000002) ; National Natural Science Foundation of China(51306189) ; Science and Technology Program of Guangdong Province(2014A010106022) ; Comprehensive Strategic Cooperation Project of Guangdong Province ; Chinese Academy of Sciences(2012B090400042) ; China-EU SMEs Cooperation Fund for Energy Conservation Research Project(SQ2013ZOB000002)
DOI10.1007/s10562-016-1877-4
研究领域[WOS]Chemistry
关键词[WOS]ACETIC-ACID ; CO ADSORPTION ; LACTIC-ACID ; RUTHENIUM CATALYSTS ; SUCCINIC ACID ; HYDROGENATION ; BIOMASS ; HYDROGENOLYSIS ; REDUCTION ; CHEMICALS
收录类别SCI
语种英语
资助者National Natural Science Foundation of China(51306189) ; Science and Technology Program of Guangdong Province(2014A010106022) ; Comprehensive Strategic Cooperation Project of Guangdong Province ; Chinese Academy of Sciences(2012B090400042) ; China-EU SMEs Cooperation Fund for Energy Conservation Research Project(SQ2013ZOB000002) ; National Natural Science Foundation of China(51306189) ; Science and Technology Program of Guangdong Province(2014A010106022) ; Comprehensive Strategic Cooperation Project of Guangdong Province ; Chinese Academy of Sciences(2012B090400042) ; China-EU SMEs Cooperation Fund for Energy Conservation Research Project(SQ2013ZOB000002)
WOS类目Chemistry, Physical
WOS记录号WOS:000394139200004
引用统计
被引频次:1[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/14047
专题中国科学院广州能源研究所
作者单位Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
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GB/T 7714
Chen, Lungang,Li, Yuping,Zhang, Xinghua,et al. Effect of Ru Particle Size on Hydrogenation/Decarbonylation of Propanoic Acid Over Supported Ru Catalysts in Aqueous Phase[J]. CATALYSIS LETTERS,2017,147(1):29-38.
APA Chen, Lungang,Li, Yuping,Zhang, Xinghua,Zhang, Qi,Wang, Tiejun,&Ma, Longlong.(2017).Effect of Ru Particle Size on Hydrogenation/Decarbonylation of Propanoic Acid Over Supported Ru Catalysts in Aqueous Phase.CATALYSIS LETTERS,147(1),29-38.
MLA Chen, Lungang,et al."Effect of Ru Particle Size on Hydrogenation/Decarbonylation of Propanoic Acid Over Supported Ru Catalysts in Aqueous Phase".CATALYSIS LETTERS 147.1(2017):29-38.
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