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Hydrogen production from bio-oil model compounds dry (CO2) reforming over Ni/Al2O3 catalyst
Fu, Ming1; Qi, Wei2; Xu, Qingli1; Zhang, Suping1; Yan, Yongjie1
2016-01-21
发表期刊INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
卷号41期号:3页码:1494-1501
摘要Bio-oil model compounds dry (CO2) reforming for hydrogen production over Ni/Al2O3 catalyst is presented in this paper. The research investigates the effects of reaction conditions such as temperature, weight hourly space velocity of the aqueous phase (WHSV), CO2 to carbon in bio-oil ratio (CO2/Bio-oil) on hydrogen yield and products distribution. And also study the coke formation rates versus different reaction temperature and different CO2/Bio-oil ratio. Meanwhile analyze the types of carbon deposited on Ni/Al2O3 catalyst. The experimental results show that, the optimum reaction temperature is 700 degrees C, CO2/Bio-oil is 0.75, WHSV is 0.9 h(-1), under these conditions, hydrogen yield and bio-oil model compounds conversion reach 88.19% and 96.87% respectively, the molar ratio of H-2/CO reaches 1.08. The coke formation rate exists a maximum at 600 degrees C, higher temperature (>600 degrees C) and higher CO2/Bio-oil (>0.75) are all good for carbon elimination of dry reforming. The forms of carbon deposit on Ni/Al2O3 catalyst are mainly filamentous carbon and graphitic carbon. Copyright (c) 2015, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
文章类型Article
关键词Dry Reforming Bio-oil Hydrogen Carbon Deposition
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.ijhydene.2015.11.104
研究领域[WOS]Chemistry ; Electrochemistry ; Energy & Fuels
关键词[WOS]BIOMASS STEAM GASIFICATION ; NOBLE-METAL CATALYSTS ; SUPERCRITICAL WATER ; SYNGAS PRODUCTION ; GAS-PRODUCTION ; BED REACTOR ; ACETIC-ACID ; RICH GAS ; COAL ; CH4
收录类别SCI
语种英语
WOS类目Chemistry, Physical ; Electrochemistry ; Energy & Fuels
WOS记录号WOS:000369461500013
引用统计
被引频次:5[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/11012
专题中国科学院广州能源研究所
作者单位1.E China Univ Sci & Technol, Minist Educ, Key Lab Coal Gasificat & Energy Chem Engn, Res Ctr Biomass Energy, Shanghai 200237, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou, Guangdong, Peoples R China
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Fu, Ming,Qi, Wei,Xu, Qingli,et al. Hydrogen production from bio-oil model compounds dry (CO2) reforming over Ni/Al2O3 catalyst[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2016,41(3):1494-1501.
APA Fu, Ming,Qi, Wei,Xu, Qingli,Zhang, Suping,&Yan, Yongjie.(2016).Hydrogen production from bio-oil model compounds dry (CO2) reforming over Ni/Al2O3 catalyst.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,41(3),1494-1501.
MLA Fu, Ming,et al."Hydrogen production from bio-oil model compounds dry (CO2) reforming over Ni/Al2O3 catalyst".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 41.3(2016):1494-1501.
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