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Selective Conversion of Cellulose into Ethylene Glycol over Metal-Organic Framework-Derived Multifunctional Catalysts
Wang, Shengpei1,2; Chen, Jinzhu1; Chen, Limin3
2014-10-01
发表期刊CATALYSIS LETTERS
卷号144期号:10页码:1728-1734
摘要A multifunctional catalyst of ruthenium supported on NENU-3 [a hybrid of phosphotungstic acid (PTA) and HKUST-1] is developed. An ethylene glycol (EG) yield of 50.2 % can be directly obtained from cellulose with Ru/NENU-3 as catalyst under optimized conditions. As a multifunctional catalyst of Ru/NENU-3, the presence of both the active specie of PTA for cellulose hydrolysis and subsequent C-C bond cleavage of cellulose-derived sugars, and the active specie of Ru for glycolaldehyde hydrogenation is indispensible for the formation of EG from cellulose.
文章类型Article
关键词Cellulose Ethylene Glycol Metal-organic Frameworks Multifunctional Catalyst Ruthenium
WOS标题词Science & Technology ; Physical Sciences
DOI10.1007/s10562-014-1334-1
研究领域[WOS]Chemistry
关键词[WOS]TUNGSTEN CARBIDE CATALYSTS ; BIMETALLIC CATALYSTS ; SUGAR ALCOHOLS ; BIOMASS ; CHEMICALS ; FUELS ; ACID ; NI
收录类别SCI
语种英语
WOS类目Chemistry, Physical
WOS记录号WOS:000341859600011
引用统计
被引频次:5[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10770
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.S China Univ Technol, Coll Environm & Energy, Guangzhou 510006, Guangdong, Peoples R China
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GB/T 7714
Wang, Shengpei,Chen, Jinzhu,Chen, Limin. Selective Conversion of Cellulose into Ethylene Glycol over Metal-Organic Framework-Derived Multifunctional Catalysts[J]. CATALYSIS LETTERS,2014,144(10):1728-1734.
APA Wang, Shengpei,Chen, Jinzhu,&Chen, Limin.(2014).Selective Conversion of Cellulose into Ethylene Glycol over Metal-Organic Framework-Derived Multifunctional Catalysts.CATALYSIS LETTERS,144(10),1728-1734.
MLA Wang, Shengpei,et al."Selective Conversion of Cellulose into Ethylene Glycol over Metal-Organic Framework-Derived Multifunctional Catalysts".CATALYSIS LETTERS 144.10(2014):1728-1734.
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