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High-performance PdRu bimetallic catalyst supported on mesoporous silica nanoparticles for phenol hydrogenation
Huang, Chao1,2; Yang, Xu3; Yang, Hui1,2; Huang, Peiyan1,2; Song, Huiyu1,2; Liao, Shijun1,2
2014-10-01
发表期刊APPLIED SURFACE SCIENCE
卷号315页码:138-143
摘要A high-performance PdRu bimetallic catalyst supported on mesoporous silica nanoparticles (MSN), PdRu/MSN, was prepared by a facile impregnation-hydrogen reduction method. It was found that PdRu/MSN showed 5 times higher activity than that of Pd/MSN towards the liquid-phase hydrogenation of phenol. The catalysts were characterized comprehensively by multiple techniques, X-ray diffraction (XRD), transmission electron microscopy (TEM), X-ray photoelectron spectroscopy (XPS), and hydrogen temperature program reduction (TPR). It was revealed that adding Ru could effectively improve the Pd dispersion and promote the electronic interaction between the Pd and Ru, both of which contribute to enhancing the catalytic activity. (C) 2014 Elsevier B.V. All rights reserved.
文章类型Article
关键词Promotion Effect Pd Ru Mesoporous Silica Phenol Hydrogenation
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.apsusc.2014.07.011
研究领域[WOS]Chemistry ; Materials Science ; Physics
关键词[WOS]SELECTIVE HYDROGENATION ; CARBON NANOTUBES ; PALLADIUM NANOPARTICLES ; ETHANOL OXIDATION ; ACETYLENE ; AG ; AROMATICS ; AL2O3 ; ACID ; FUEL
收录类别SCI
语种英语
WOS类目Chemistry, Physical ; Materials Science, Coatings & Films ; Physics, Applied ; Physics, Condensed Matter
WOS记录号WOS:000342360300021
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被引频次:16[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10753
专题中国科学院广州能源研究所
作者单位1.S China Univ Technol, Sch Chem & Chem Engn, Key Lab Fuel Cell Technol Guangdong Prov, Guangzhou, Guangdong, Peoples R China
2.S China Univ Technol, Sch Chem & Chem Engn, Key Lab New Energy Guangdong Univ, Guangzhou, Guangdong, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou, Guangdong, Peoples R China
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Huang, Chao,Yang, Xu,Yang, Hui,et al. High-performance PdRu bimetallic catalyst supported on mesoporous silica nanoparticles for phenol hydrogenation[J]. APPLIED SURFACE SCIENCE,2014,315:138-143.
APA Huang, Chao,Yang, Xu,Yang, Hui,Huang, Peiyan,Song, Huiyu,&Liao, Shijun.(2014).High-performance PdRu bimetallic catalyst supported on mesoporous silica nanoparticles for phenol hydrogenation.APPLIED SURFACE SCIENCE,315,138-143.
MLA Huang, Chao,et al."High-performance PdRu bimetallic catalyst supported on mesoporous silica nanoparticles for phenol hydrogenation".APPLIED SURFACE SCIENCE 315(2014):138-143.
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