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Production of Hydrocarbons via Hydrodeoxygenation of Lignin-Derived Phenolic Compounds
Zhang Xinghua; Chen Lungang; Zhang Qi; Long Jinxing; Wang Tiejun; Ma Longlong
2014-12-01
Source PublicationPROGRESS IN CHEMISTRY
Volume26Issue:12Pages:1997-2006
AbstractLignin is the component with the highest carbon content in biomass. The transformation of lignin to high-grade liquid fuels can be achieved via hydrodeoxygenation(HDO) of phenolic intermediates derived from the products of lignin depolymerization. The octane numbers of the hydrodeoxygenation products of phenolic intermediates are quite high. They have vapor pressures and carbon atom number (C6 similar to C10) within the range of gasoline. Thus, these hydrodeoxygenation products would be the most desirable components for a fungible liquid transportation fuel. This is very meaningful to application of lignin. Recently, researches about the hydrodeoxygenation of phenolic compounds develop rapidly. In this paper, the HDO reactions of phenolic compounds using sulfided Mo-based catalyst, noble metal catalyst and inexpensive non-sulfided catalyst are reviewed in detail. It is found that most of the investigated catalysts are bifunctional catalysts, combining the hydrogenation function of active metal with hydrolysis and dehydration of support. The catalytic mechanism for the HDO of phenolic compounds is sketched, and the effects of catalyst supporter on the catalytic activity are also discussed. Furthermore, the current technique challenges are summarized, and future technologic explorations for the efficient hydrodeoxygenation of lignin-derived phenolic compounds are proposed.
SubtypeArticle
KeywordLignin Phenolic Compounds Hydrocarbons Hydrodeoxygenation Active Metal Supporter
WOS HeadingsScience & Technology ; Physical Sciences
DOI10.7536/PC140815
WOS Subject ExtendedChemistry
WOS KeywordB AMORPHOUS CATALYSTS ; NOBLE-METAL CATALYSTS ; NI-BASED CATALYSTS ; BIO-OIL ; PYROLYSIS OIL ; HYDRODESULFURIZATION CATALYSTS ; SUPPORTED PALLADIUM ; GUAIACOL HYDRODEOXYGENATION ; SULFIDED COMO/GAMMA-AL2O3 ; SELECTIVE HYDROGENATION
Indexed BySCI
Language英语
WOS SubjectChemistry, Multidisciplinary
WOS IDWOS:000348006500010
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Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/10742
Collection中国科学院广州能源研究所
AffiliationChinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
Recommended Citation
GB/T 7714
Zhang Xinghua,Chen Lungang,Zhang Qi,et al. Production of Hydrocarbons via Hydrodeoxygenation of Lignin-Derived Phenolic Compounds[J]. PROGRESS IN CHEMISTRY,2014,26(12):1997-2006.
APA Zhang Xinghua,Chen Lungang,Zhang Qi,Long Jinxing,Wang Tiejun,&Ma Longlong.(2014).Production of Hydrocarbons via Hydrodeoxygenation of Lignin-Derived Phenolic Compounds.PROGRESS IN CHEMISTRY,26(12),1997-2006.
MLA Zhang Xinghua,et al."Production of Hydrocarbons via Hydrodeoxygenation of Lignin-Derived Phenolic Compounds".PROGRESS IN CHEMISTRY 26.12(2014):1997-2006.
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