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Hydrogen production by steam reforming of dimethyl ether and CO-PrOx in a metal foam micro-reactor
Yan, Changfeng1,2; Hai, Hang2; Guo, Changqing1; Li, Wenbo1; Huang, Shilin1; Chen, Hao1
2014-07-03
发表期刊INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
卷号39期号:20页码:10409-10416
摘要A bi-function catalyst containing CuZnAlCr and HZSM-5 was used to generate hydrogen by stream reforming of dimethyl ether (SRD) in a metal foam micro-reactor and a fix-bed reactor. Dimethyl ether conversion of 99% and hydrogen yield of >95% was reached with HZSM-5/CuZnAlCr (mass ratio of 1:1) in the micro-reactor. A suitable balance between the dimethyl ether hydrolysis and methanol reforming steps requires the proper acidity and the metal sites. The CuZnAlCr/HZSM-5 properties, effect of CuZnAlCr to HZSM-5 mass ratio were investigated in the metal foam micro-reactor. Moreover, CO was removed from hydrogen-rich gas by preferential oxidation reaction (CO-PrOx) with PtFe/gamma-Al2O3 catalyst in a similar metal foam micro-reactor follows the SRD stage. With the optimized O-2/CO ratio and reaction temperature, the CO concentration dropped to <10 ppm and hydrogen yield of similar to 90% were achieved in the new-type SRD-COPrOx system. The SRD-COPrOx system provide a constant hydrogen production with CO concentration lower than 10 ppm during 20 h. The results indicate that metal foam micro-reactor has the great potential in the DME steam reforming to supply hydrogen for low-temperature fuel cells. Copyright (C) 2014, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
文章类型Article
关键词Metal Foam Hydrogen Production Dme Steam Reforming Micro-reactor
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.ijhydene.2014.04.096
研究领域[WOS]Chemistry ; Electrochemistry ; Energy & Fuels
关键词[WOS]FUEL-CELLS ; MICROCHANNEL REACTOR ; COMPOSITE CATALYSTS ; NICKEL-CATALYSTS ; CARBON FORMATION ; FLUIDIZED-BED ; NOBLE-METAL ; METHANOL ; OXIDATION ; ETHANOL
收录类别SCI
语种英语
WOS类目Chemistry, Physical ; Electrochemistry ; Energy & Fuels
WOS记录号WOS:000338388200009
引用统计
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10690
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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Yan, Changfeng,Hai, Hang,Guo, Changqing,et al. Hydrogen production by steam reforming of dimethyl ether and CO-PrOx in a metal foam micro-reactor[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2014,39(20):10409-10416.
APA Yan, Changfeng,Hai, Hang,Guo, Changqing,Li, Wenbo,Huang, Shilin,&Chen, Hao.(2014).Hydrogen production by steam reforming of dimethyl ether and CO-PrOx in a metal foam micro-reactor.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,39(20),10409-10416.
MLA Yan, Changfeng,et al."Hydrogen production by steam reforming of dimethyl ether and CO-PrOx in a metal foam micro-reactor".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 39.20(2014):10409-10416.
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