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Kinetic Behaviors of Methane Hydrate Formation in Porous Media in Different Hydrate Deposits
Li, Bo1,2,3; Li, Xiao-Sen1,2; Li, Gang1,2; Wang, Yi1,2; Feng, Jing-Chun1,2,3
2014-04-02
Source PublicationINDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
Volume53Issue:13Pages:5464-5474
AbstractThe kinetic characteristics of methane hydrate formation in porous media are investigated in three experimental apparatus with different scales. A total of 18 experimental formation runs are implemented in these apparatus (6 runs in each device). The kinetic model proposed by Li et al. [Chem. Eng. Sci., 2014, 105, 220-230] is employed to simulate these hydrate formation processes, and the applicability of this model in different hydrate deposits is confirmed by comparing the experimental data with the numerical prediction. It is found that the reaction rate constant k decreases sharply with the increase of the size of the apparatus, which indicates that the hydrate formation rate is inversely proportional to the scale of the hydrate deposit. In addition, both the initial phase saturations and the properties of the porous media show extraordinary effects on the formation kinetics of methane hydrate.
SubtypeArticle
WOS HeadingsScience & Technology ; Technology
DOI10.1021/ie500580y
WOS Subject ExtendedEngineering
WOS KeywordSINGLE HORIZONTAL WELL ; COAL-MINE GAS ; PUFF METHOD ; NUMERICAL-SIMULATION ; QILIAN MOUNTAIN ; CRYSTALLIZATION ; SEPARATION ; DEPRESSURIZATION ; DIOXIDE ; GROWTH
Indexed BySCI
Language英语
WOS SubjectEngineering, Chemical
WOS IDWOS:000333947600041
Citation statistics
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/10667
Collection中国科学院广州能源研究所
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou 510640, Guangdong, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100083, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Li, Bo,Li, Xiao-Sen,Li, Gang,et al. Kinetic Behaviors of Methane Hydrate Formation in Porous Media in Different Hydrate Deposits[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2014,53(13):5464-5474.
APA Li, Bo,Li, Xiao-Sen,Li, Gang,Wang, Yi,&Feng, Jing-Chun.(2014).Kinetic Behaviors of Methane Hydrate Formation in Porous Media in Different Hydrate Deposits.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,53(13),5464-5474.
MLA Li, Bo,et al."Kinetic Behaviors of Methane Hydrate Formation in Porous Media in Different Hydrate Deposits".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 53.13(2014):5464-5474.
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