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Kinetic Behaviors of Methane Hydrate Formation in Porous Media in Different Hydrate Deposits
Li, Bo1,2,3; Li, Xiao-Sen1,2; Li, Gang1,2; Wang, Yi1,2; Feng, Jing-Chun1,2,3
2014-04-02
发表期刊INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
卷号53期号:13页码:5464-5474
摘要The kinetic characteristics of methane hydrate formation in porous media are investigated in three experimental apparatus with different scales. A total of 18 experimental formation runs are implemented in these apparatus (6 runs in each device). The kinetic model proposed by Li et al. [Chem. Eng. Sci., 2014, 105, 220-230] is employed to simulate these hydrate formation processes, and the applicability of this model in different hydrate deposits is confirmed by comparing the experimental data with the numerical prediction. It is found that the reaction rate constant k decreases sharply with the increase of the size of the apparatus, which indicates that the hydrate formation rate is inversely proportional to the scale of the hydrate deposit. In addition, both the initial phase saturations and the properties of the porous media show extraordinary effects on the formation kinetics of methane hydrate.
文章类型Article
WOS标题词Science & Technology ; Technology
DOI10.1021/ie500580y
研究领域[WOS]Engineering
关键词[WOS]SINGLE HORIZONTAL WELL ; COAL-MINE GAS ; PUFF METHOD ; NUMERICAL-SIMULATION ; QILIAN MOUNTAIN ; CRYSTALLIZATION ; SEPARATION ; DEPRESSURIZATION ; DIOXIDE ; GROWTH
收录类别SCI
语种英语
WOS类目Engineering, Chemical
WOS记录号WOS:000333947600041
引用统计
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10667
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou 510640, Guangdong, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100083, Peoples R China
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Li, Bo,Li, Xiao-Sen,Li, Gang,et al. Kinetic Behaviors of Methane Hydrate Formation in Porous Media in Different Hydrate Deposits[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2014,53(13):5464-5474.
APA Li, Bo,Li, Xiao-Sen,Li, Gang,Wang, Yi,&Feng, Jing-Chun.(2014).Kinetic Behaviors of Methane Hydrate Formation in Porous Media in Different Hydrate Deposits.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,53(13),5464-5474.
MLA Li, Bo,et al."Kinetic Behaviors of Methane Hydrate Formation in Porous Media in Different Hydrate Deposits".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 53.13(2014):5464-5474.
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