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Research on in situ Hydrogenation of o-Cresol over Ni/CMK-3 Catalysts
Li Yanbin1,2; Xu Ying2,3; Ma Longlong1,2,3; Zhang Qi2,3; Wang Tiejun2,3; Chen Guanyi1; Zhang Limin2
2014-12-10
发表期刊CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE
卷号35期号:12页码:2654-2661
摘要In situ hydrogenation was studied by means of Ni loading, temperature, initial pressure, and reaction time over Ni/CMK-3 catalysts. The catalysts were characterized by X-ray diffraction(XRD), H-2 temperature programmed reduction(H-2-TPR) and N-2 adsorption-desorption isotherms. The results revealed that the optimal conditions were confirmed as follow: Ni loading of 20% (mass fraction), reaction temperature of 230 degrees C, initial pressure of 0. 1 MPa, reaction time of 9 h for in situ hydrogenation. The maximum conversion of o-cresol in optimal condition was determined as 47. 56%. Compared with the effect of hydrogen donor solvents, formic acid was the best of four kinds of solvents. The comparsion of cresol isomers, recyclability of Ni/CMK-3 were also discussed.
文章类型Article
关键词In Situ Hydrogenation O-cresol Nickel-based Cmk-3 Catalyst
WOS标题词Science & Technology ; Physical Sciences
DOI10.7503/cjcu20140464
研究领域[WOS]Chemistry
关键词[WOS]OIL MODEL COMPOUNDS ; BIO-OIL ; PLATINUM CATALYSTS ; GENERATED HYDROGEN ; MESOPOROUS CARBONS ; PYROLYSIS OIL ; HYDRODEOXYGENATION ; PHENOL ; PERFORMANCE ; COMPOUND
收录类别SCI
语种英语
WOS类目Chemistry, Multidisciplinary
WOS记录号WOS:000347669400025
引用统计
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10643
专题中国科学院广州能源研究所
作者单位1.Tianjin Univ, State Key Lab Int Combust Engine, Fac Environm Sci & Engn, Tianjin 300072, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
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Li Yanbin,Xu Ying,Ma Longlong,et al. Research on in situ Hydrogenation of o-Cresol over Ni/CMK-3 Catalysts[J]. CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,2014,35(12):2654-2661.
APA Li Yanbin.,Xu Ying.,Ma Longlong.,Zhang Qi.,Wang Tiejun.,...&Zhang Limin.(2014).Research on in situ Hydrogenation of o-Cresol over Ni/CMK-3 Catalysts.CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,35(12),2654-2661.
MLA Li Yanbin,et al."Research on in situ Hydrogenation of o-Cresol over Ni/CMK-3 Catalysts".CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE 35.12(2014):2654-2661.
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