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Phase Equilibrium Data of the Double Tetrabutylammonium Chloride Plus Carbon Dioxide or Nitrogen Semiclathrate Hydrate
Shi, Ling-Li1,2; Liang, De-Qing1; Wu, Neng-You1
2014-07-01
Source PublicationJOURNAL OF CHEMICAL AND ENGINEERING DATA
Volume59Issue:7Pages:2320-2323
AbstractIn this paper, phase equilibrium data of the double tetrabutylammonium chloride (TBACl: C16H36ClN) semidathrate hydrate with a guest gas (CO2 or N-2) at four different TBACl concentrations (0.06, 0.15, 0.34, and 0.44 mass fraction) were experimentally measured by employing an isochoric pressure-search method in the temperature range of (282.9 to 293.2) K and at pressures up to 13.57 MPa, respectively. The results demonstrated that double TBACl + CO2 (or N-2) semidathrate hydrates had an obvious advantage in thermal stability compared to pure CO2 (or N-2) hydrates. And the strongest stabilization effect was observed with the application of TBACl at 0.34 mass fraction, corresponding to TBACl center dot 30H(2)O. In addition, the results were compared with the corresponding data reported in open literature. The comparisons showed that some literature data seemed to be not reliable.
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1021/je500445w
WOS Subject ExtendedChemistry ; Engineering
WOS KeywordN-BUTYLAMMONIUM BROMIDE ; DISSOCIATION CONDITIONS ; AMMONIUM-CHLORIDE ; WATER ; CO2 ; HYDROGEN ; METHANE ; MIXTURES ; BINARY ; SYSTEM
Indexed BySCI
Language英语
WOS SubjectChemistry, Multidisciplinary ; Engineering, Chemical
WOS IDWOS:000338981000025
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Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/10602
Collection中国科学院广州能源研究所
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Shi, Ling-Li,Liang, De-Qing,Wu, Neng-You. Phase Equilibrium Data of the Double Tetrabutylammonium Chloride Plus Carbon Dioxide or Nitrogen Semiclathrate Hydrate[J]. JOURNAL OF CHEMICAL AND ENGINEERING DATA,2014,59(7):2320-2323.
APA Shi, Ling-Li,Liang, De-Qing,&Wu, Neng-You.(2014).Phase Equilibrium Data of the Double Tetrabutylammonium Chloride Plus Carbon Dioxide or Nitrogen Semiclathrate Hydrate.JOURNAL OF CHEMICAL AND ENGINEERING DATA,59(7),2320-2323.
MLA Shi, Ling-Li,et al."Phase Equilibrium Data of the Double Tetrabutylammonium Chloride Plus Carbon Dioxide or Nitrogen Semiclathrate Hydrate".JOURNAL OF CHEMICAL AND ENGINEERING DATA 59.7(2014):2320-2323.
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