GIEC OpenIR  > 中国科学院广州能源研究所
Effect of iron promoter on structure and performance of CuMnZnO catalyst for higher alcohols synthesis
Ding, Mingyue1,2; Qiu, Minghuang1,2,3; Wang, Tiejun1,2; Ma, Longlong1,2; Wu, Chuangzhi1,2; Liu, Jianguo1,2,3
2012-09-01
发表期刊APPLIED ENERGY
卷号97页码:543-547
摘要Effect of iron promoter on the microstructures of CuMnZnO catalysts was investigated by N-2 physical adsorption (BET), X-ray diffraction (XRD), and temperature-programmed reduction of hydrogen (H-2-TPR). Higher alcohols synthesis (HAS) was performed in a fixed bed reactor. The characterization results indicated that incorporation of iron in the CuMnZnO catalyst resulted in the increase of BET surface area and the dispersion of catalyst particles. Adding iron facilitated the formation of Fe-Mn solid solution and reduced the interaction between copper and manganese, which promoted the separation of CuO from the Cu-Mn solid solution and the reduction of the catalyst. In the HAS reaction, the catalytic activity of CO hydrogenation and the selectivity to C;OH and hydrocarbons presented an increasing trend with the increase in iron concentration, which may be attributed to the synergistic effect between the dispersed copper and iron carbides. (C) 2011 Elsevier Ltd. All rights reserved.
文章类型Article
关键词Higher Alcohol Synthesis Iron Promoter Cumnzno Catalyst Synergistic Effect
WOS标题词Science & Technology ; Technology
DOI10.1016/j.apenergy.2011.11.083
研究领域[WOS]Energy & Fuels ; Engineering
关键词[WOS]FISCHER-TROPSCH SYNTHESIS ; K2CO3/MOS2 CATALYST ; SYNGAS ; COPPER ; CO ; CONVERSION ; ETHANOL ; BIOFUELS ; BIOMASS
收录类别SCI ; ISTP
语种英语
WOS类目Energy & Fuels ; Engineering, Chemical
WOS记录号WOS:000307196000063
引用统计
被引频次:20[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10587
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Key Lab Renewable Energy & Nat Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
3.Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Ding, Mingyue,Qiu, Minghuang,Wang, Tiejun,et al. Effect of iron promoter on structure and performance of CuMnZnO catalyst for higher alcohols synthesis[J]. APPLIED ENERGY,2012,97:543-547.
APA Ding, Mingyue,Qiu, Minghuang,Wang, Tiejun,Ma, Longlong,Wu, Chuangzhi,&Liu, Jianguo.(2012).Effect of iron promoter on structure and performance of CuMnZnO catalyst for higher alcohols synthesis.APPLIED ENERGY,97,543-547.
MLA Ding, Mingyue,et al."Effect of iron promoter on structure and performance of CuMnZnO catalyst for higher alcohols synthesis".APPLIED ENERGY 97(2012):543-547.
条目包含的文件
条目无相关文件。
个性服务
推荐该条目
保存到收藏夹
查看访问统计
导出为Endnote文件
谷歌学术
谷歌学术中相似的文章
[Ding, Mingyue]的文章
[Qiu, Minghuang]的文章
[Wang, Tiejun]的文章
百度学术
百度学术中相似的文章
[Ding, Mingyue]的文章
[Qiu, Minghuang]的文章
[Wang, Tiejun]的文章
必应学术
必应学术中相似的文章
[Ding, Mingyue]的文章
[Qiu, Minghuang]的文章
[Wang, Tiejun]的文章
相关权益政策
暂无数据
收藏/分享
所有评论 (0)
暂无评论
 

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。