Synthesis Gas Production by Chemical-Looping Reforming of Methane Using Lattice Oxygen

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	Synthesis Gas Production by Chemical-Looping Reforming of Methane Using Lattice Oxygen
	Huang Zhen; He Fang; Zhao Kun; Zheng Anqing; Li Haibin; Zhao Zengli
	2012-08-24
发表期刊	PROGRESS IN CHEMISTRY
卷号	24 期号:8 页码:1599-1609
摘要	Chemical looping reforming (CLR) of methane to obtain synthesis gas using lattice oxygen of oxygen carriers instead of molecular oxygen is a novel technology for producing synthesis gas from methane, which has higher economic benefits and environmental benign. CLR has several advantages, such as, saving oxygen generation equipment, capable of self-heating, suitable hydrogen/carbon ratio, useful by-products and realizing industrialization easily, so, it has been growing interest for researchers at home and aboard. Firstly, the basic concept and characteristics of CLR are introduced, which is partial oxidation of methane through controlling the value of lattice oxygen/fuel, thus, the synthesis gas is produced through the gas-solid reaction between methane and oxygen carriers, and the reduced oxygen carriers are re-oxidized by air or H2O to restore its lattice oxygen. Direct contact between fuel and combustion air is avoided in the CLR. Instead, an oxygen carrier performs the task of bringing O-2 from the air to the fuel. In particular, it is summarized for the research progress of monometallic and composite metal oxygen carriers. And the same time, several kinds of typical representative reactor in CLR are discussed, among which interconnected fluidized bed reactor will be most effective for CLR to realize industrialization in the future. Finally, the expand application of CLR and the trends coupled with other technology are prospected.
文章类型	Article
关键词	Methane Chemical Looping Reforming Synthesis Gas Lattice Oxygen Reactor
WOS标题词	Science & Technology ; Physical Sciences
研究领域[WOS]	Chemistry
关键词[WOS]	FLUIDIZED-BED REACTOR ; SUPPORTED NI CATALYSTS ; PARTIAL OXIDATION ; HYDROGEN-PRODUCTION ; CERIUM OXIDE ; METAL-OXIDES ; CO2 CAPTURE ; COMBUSTION ; CARRIERS ; GENERATION
收录类别	SCI
语种	英语
WOS类目	Chemistry, Multidisciplinary
WOS记录号	WOS:000308508600019
引用统计	被引频次：18[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.giec.ac.cn/handle/344007/10586
专题	中国科学院广州能源研究所
作者单位	Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Peoples R China
推荐引用方式 GB/T 7714	Huang Zhen,He Fang,Zhao Kun,et al. Synthesis Gas Production by Chemical-Looping Reforming of Methane Using Lattice Oxygen[J]. PROGRESS IN CHEMISTRY,2012,24(8):1599-1609.
APA	Huang Zhen,He Fang,Zhao Kun,Zheng Anqing,Li Haibin,&Zhao Zengli.(2012).Synthesis Gas Production by Chemical-Looping Reforming of Methane Using Lattice Oxygen.PROGRESS IN CHEMISTRY,24(8),1599-1609.
MLA	Huang Zhen,et al."Synthesis Gas Production by Chemical-Looping Reforming of Methane Using Lattice Oxygen".PROGRESS IN CHEMISTRY 24.8(2012):1599-1609.