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Mixed alcohols synthesis from syngas over activated palygorskite supported Cu-Fe-Co based catalysts
Guo, Haijun1,2; Zhang, Hairong1,2; Peng, Fen1,2; Yang, Huijuan1,2,3; Xiong, Lian1,2; Huang, Chao1,2; Wang, Can1,2; Chen, Xinde1,2; Ma, Longlong1,2
2015-07-01
发表期刊APPLIED CLAY SCIENCE
卷号111页码:83-89
摘要Conversion of lignocellulosic biomass to liquid fuels through the synthesis gas (syngas) intermediate product will become an important route for production of clean fuel in the future. In this work, H2SO4-activated palygorskite (Pal) supported Cu-Fe-Co based catalysts were prepared by an impregnation method and applied to mixed alcohols synthesis (MAS) from syngas. The structural properties of those catalysts were characterized by N-2 adsorption/desorption, X-ray diffraction (XRD), X-ray fluorescence (XRF), X-ray photoelectron spectroscopy (XPS), Scanning Electron Microscope (SEM), Transmission electron microscopy (TEM) and H-2-Temperature programmed reduction (H-2-TPR). The CFCK/Pal-B21 catalyst exhibited better catalytic activity, yield and selectivity for mixed alcohols due to the high surface concentration of Cu-FeCx dual site and the ideal interaction between Cu and Fe species. Due to the unique property and the low cost and easy availability, the Pal clay has a great promise to be used as catalyst support for liquid biofuel production from biomass-derived syngas. (C) 2015 Elsevier B.V. All rights reserved.
文章类型Article
关键词Syngas Mixed Alcohols Synthesis Palygorskite Cu-fe-co Based Catalyst
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.clay.2015.03.009
研究领域[WOS]Chemistry ; Materials Science ; Mineralogy
关键词[WOS]BIMETALLIC NANOPARTICLES ; SURFACE-PROPERTIES ; ATTAPULGITE CLAY ; CONVERSION ; BIOMASS ; HYDROGENATION ; EVOLUTION ; OXIDATION ; KINETICS ; COPPER
收录类别SCI
语种英语
WOS类目Chemistry, Physical ; Materials Science, Multidisciplinary ; Mineralogy
WOS记录号WOS:000355362600011
引用统计
被引频次:20[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10501
专题中国科学院广州能源研究所
集成技术研发中心
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, R&D Ctr Xuyi Attapulgite Appl Technol, Guangzhou 211700, Guangdong, Peoples R China
3.Chinese Acad Sci, Grad Univ, Being 100049, Peoples R China
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Guo, Haijun,Zhang, Hairong,Peng, Fen,et al. Mixed alcohols synthesis from syngas over activated palygorskite supported Cu-Fe-Co based catalysts[J]. APPLIED CLAY SCIENCE,2015,111:83-89.
APA Guo, Haijun.,Zhang, Hairong.,Peng, Fen.,Yang, Huijuan.,Xiong, Lian.,...&Ma, Longlong.(2015).Mixed alcohols synthesis from syngas over activated palygorskite supported Cu-Fe-Co based catalysts.APPLIED CLAY SCIENCE,111,83-89.
MLA Guo, Haijun,et al."Mixed alcohols synthesis from syngas over activated palygorskite supported Cu-Fe-Co based catalysts".APPLIED CLAY SCIENCE 111(2015):83-89.
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