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A high efficient photoluminescence Zn-Cu-In-S/ZnS quantum dots with long lifetime
Wang, Xin1,2; Liang, Zhurong2,3; Xu, Xueqing2,3; Wang, Nan1,2; Fang, Jun1; Wang, Junxia2,3; Xu, Gang2,3
2015-08-15
发表期刊JOURNAL OF ALLOYS AND COMPOUNDS
卷号640页码:134-140
摘要Highly Cu-rich copper indium sulfide (CuInS2, CIS) quantum dots were synthesized utilizing copper chloride (CuCl) and indium acetate (In(Ac)(3)) as metal cation precursors, combined with n-dodecanethiol (DDT) as a coordinating sulfur source and solvent. With excess of In(Ac)(3), i.e. with Cu/In ratios of 1/4, together with Zn2+ ions post-treatment, a relatively high photoluminescence quantum yield (QY) of similar to 73% with long average lifetime of similar to 359 ns has been obtained, which is proposed to be attributed to the Cu-rich defect states in the CIS nanocrystals (NCs) nuclei. Meanwhile, the formation of In-rich CIS-ZnS alloy, i.e. Zn-Cu-In-S (ZCIS) with high density of Cu vacancies, combined with the surface passivation of ZnS overlay resulted in a high QY. Finally, the formation mechanism of the ZCIS/ZnS with Cu-rich nuclei has been proposed. (C) 2015 Elsevier B.V. All rights reserved.
文章类型Article
关键词Cuins2 Quantum Dots Photoluminescence Long Lifetime
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.jallcom.2015.03.249
研究领域[WOS]Chemistry ; Materials Science ; Metallurgy & Metallurgical Engineering
关键词[WOS]LIGHT-EMITTING-DIODES ; SEMICONDUCTOR NANOCRYSTALS ; CUINS2 NANOCRYSTALS ; OPTICAL-PROPERTIES ; NANOPARTICLES ; TERNARY ; ELECTROLUMINESCENCE ; PRECURSOR ; FILMS ; SHAPE
收录类别SCI
语种英语
WOS类目Chemistry, Physical ; Materials Science, Multidisciplinary ; Metallurgy & Metallurgical Engineering
WOS记录号WOS:000354195600022
引用统计
被引频次:56[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10496
专题中国科学院广州能源研究所
作者单位1.Xiamen Univ, Coll Chem & Chem Engn, Dept Chem & Biochem Engn, Xiamen 361005, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
第一作者单位中国科学院广州能源研究所
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Wang, Xin,Liang, Zhurong,Xu, Xueqing,et al. A high efficient photoluminescence Zn-Cu-In-S/ZnS quantum dots with long lifetime[J]. JOURNAL OF ALLOYS AND COMPOUNDS,2015,640:134-140.
APA Wang, Xin.,Liang, Zhurong.,Xu, Xueqing.,Wang, Nan.,Fang, Jun.,...&Xu, Gang.(2015).A high efficient photoluminescence Zn-Cu-In-S/ZnS quantum dots with long lifetime.JOURNAL OF ALLOYS AND COMPOUNDS,640,134-140.
MLA Wang, Xin,et al."A high efficient photoluminescence Zn-Cu-In-S/ZnS quantum dots with long lifetime".JOURNAL OF ALLOYS AND COMPOUNDS 640(2015):134-140.
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