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Hydrogen-rich gas production from biomass catalytic gasification
Lv, PM; Chang, J; Wang, TJ; Fu, Y; Chen, Y; Zhu, JX
2004
发表期刊ENERGY & FUELS
卷号18期号:1页码:228-233
摘要With the use of dolomite in the fluidized-bed gasifier and the use of nickel-based catalysts in the fixed bed reactor downstream from the gasifier, the characteristics of hydrogen yield from biomass are investigated in the present study. Some calcined dolomite is placed initially in the gasifier with an amount of 120 g/(kg h(-1)) biomass. To replace the eroded and elutriated dolomite, calcined dolomite (0.3-0.45 mm) is continuously fed and its feeding rate is determined by preliminary test. The influence of the operating conditions in the catalytic reactor on the production of gases, especially H-2, is studied over the temperature range of 650-850 degreesC, for weight hourly space velocity (WHSV) in the range of 2.68-10.72 h(-1). In the gaseous product, the average content of H-2 exceeds 50 vol %; C-2 content is lowered to below 1 vol %, and nearly half of CH4 is converted after the catalytic reactor. Over the ranges of experimental conditions examined, the highest gas yield reaches 3.31 Nm(3)/kg biomass, wet basis; the maximum hydrogen yield reaches 130.28 g H-2/kg biomass, wet basis. This system shows a good performance over a lifetime test of 350 min.
文章类型Article
WOS标题词Science & Technology ; Technology
DOI10.1021/ef0301203
研究领域[WOS]Energy & Fuels ; Engineering
关键词[WOS]STEAM REFORMING CATALYSTS ; FLUIDIZED-BED ; HOT GAS ; OXYGEN MIXTURES ; RAW GAS ; AIR ; DOLOMITE
收录类别SCI
语种英语
WOS类目Energy & Fuels ; Engineering, Chemical
WOS记录号WOS:000188415000028
引用统计
被引频次:57[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10475
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510070, Peoples R China
2.Univ Western Ontario, London, ON N6A 5B9, Canada
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Lv, PM,Chang, J,Wang, TJ,et al. Hydrogen-rich gas production from biomass catalytic gasification[J]. ENERGY & FUELS,2004,18(1):228-233.
APA Lv, PM,Chang, J,Wang, TJ,Fu, Y,Chen, Y,&Zhu, JX.(2004).Hydrogen-rich gas production from biomass catalytic gasification.ENERGY & FUELS,18(1),228-233.
MLA Lv, PM,et al."Hydrogen-rich gas production from biomass catalytic gasification".ENERGY & FUELS 18.1(2004):228-233.
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