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Formation process and fractal growth model of HCFC-141b refrigerant gas hydrate
Zhao, YL; Guo, KH; Liang, D; Fan, SS; Liu, XC; Shu, BF; Ge, XS; Liu, Y
2002-04-01
发表期刊SCIENCE IN CHINA SERIES B-CHEMISTRY
卷号45期号:2页码:216-224
摘要The microscopic visualization experiment on the formation process of HCFC-141b refrigerant gas hydrate has been investigated, and the morphological photos of hydrate formation process have been obtained. The results show that gas hydrate originally nucleated on the interface of refrigerant HCFC-141b and water under the condition of supercooling, then the hydrate grows continually due to the inducement of formed nucleation and diffusion of refrigerant. The formation of gas hydrate presents an arboreous phenomenon. The fractal dimension of the hydrate formation morphology on different stages was calculated. The calculating results indicate that the initial stage of the hydrate formation belongs to fractal growth, and the dimension is about 1.52. Based on the fractal theory, an RIN-DLA (random inducement nucleation-diffusion limited aggregation) model for the HCFC-141b hydrate growth was developed. The hydrate growth process was simulated with the developed model, and the fractal dimension for the simulated morphology is well compared with that from the experiment.
文章类型Article
关键词Refrigerant Gas Hydrate Formation Process Fractal Growth Dimension Rin-dla Model
WOS标题词Science & Technology ; Physical Sciences
研究领域[WOS]Chemistry
收录类别SCI
语种英语
WOS类目Chemistry, Multidisciplinary
WOS记录号WOS:000175009000014
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被引频次:11[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10443
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510070, Peoples R China
2.Univ Sci & Technol China, Hefei 430070, Peoples R China
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GB/T 7714
Zhao, YL,Guo, KH,Liang, D,et al. Formation process and fractal growth model of HCFC-141b refrigerant gas hydrate[J]. SCIENCE IN CHINA SERIES B-CHEMISTRY,2002,45(2):216-224.
APA Zhao, YL.,Guo, KH.,Liang, D.,Fan, SS.,Liu, XC.,...&Liu, Y.(2002).Formation process and fractal growth model of HCFC-141b refrigerant gas hydrate.SCIENCE IN CHINA SERIES B-CHEMISTRY,45(2),216-224.
MLA Zhao, YL,et al."Formation process and fractal growth model of HCFC-141b refrigerant gas hydrate".SCIENCE IN CHINA SERIES B-CHEMISTRY 45.2(2002):216-224.
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