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Synthesis Gas from Pyrolysis of Cedar Sawdust as Biomass Materials: Characterization and Catalytic Performance of Nickel-Based Monolithic Catalyst
Lu Min1,2; Lue Pengmei1; Yuan Zhenhong1; Li Huiwen1; Xu Jingliang1
2011-06-01
发表期刊CHINESE JOURNAL OF CATALYSIS
卷号32期号:6页码:1017-1021
摘要A series of monolithic catalysts with different NiO loadings were prepared by supported on the acid treated cordierite. Their specific surface area, pore volume, pore distribution, and catalytic performance in the reforming reaction of biomass pyrolysis gas for synthesis gas were studied. The results show that the specific surface area and pore volume of the cordierite after acid treatment are up to 156 m(2)/g and 0.099 m(3)/g respectively. However, with increasing nickel oxide loading, the specific surface area and pore volume of the catalyst decrease greatly and then tend to steady. The effect of nickel oxide loading on gas composition is quite small, and the total content of H(2) and CO is maintained at 90%. The tar conversion is not affected by the specific surface area of the catalysts. After 6 h catalytic reaction, the structure of the catalysts with 28% NiO does not change, and the quantity of carbon deposition is about 1%. The tar conversion decreases from 87.4% to 81.3%. It is suggested that the nickel-based catalyst has relatively stable activity under high tar concentration conditions, which is attributed to the high dispersion of nickel particles on the support and high stability of the catalyst phase structure.
文章类型Article
关键词Biomass Synthesis Gas Cordierite Acid Treatment Nickel Oxide Tar Conversion Carbon Deposition
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.3724/SP.J.1088.2011.10139
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]FISCHER-TROPSCH SYNTHESIS ; FLUIDIZED-BED ; TAR ELIMINATION ; GASIFICATION ; STEAM ; REDUCTION ; OLIVINE ; SYNGAS ; NOX
收录类别SCI
语种英语
WOS类目Chemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
WOS记录号WOS:000292429000018
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文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10361
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
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Lu Min,Lue Pengmei,Yuan Zhenhong,et al. Synthesis Gas from Pyrolysis of Cedar Sawdust as Biomass Materials: Characterization and Catalytic Performance of Nickel-Based Monolithic Catalyst[J]. CHINESE JOURNAL OF CATALYSIS,2011,32(6):1017-1021.
APA Lu Min,Lue Pengmei,Yuan Zhenhong,Li Huiwen,&Xu Jingliang.(2011).Synthesis Gas from Pyrolysis of Cedar Sawdust as Biomass Materials: Characterization and Catalytic Performance of Nickel-Based Monolithic Catalyst.CHINESE JOURNAL OF CATALYSIS,32(6),1017-1021.
MLA Lu Min,et al."Synthesis Gas from Pyrolysis of Cedar Sawdust as Biomass Materials: Characterization and Catalytic Performance of Nickel-Based Monolithic Catalyst".CHINESE JOURNAL OF CATALYSIS 32.6(2011):1017-1021.
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