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The role of CeO(2)-ZrO(2) as support in the ZnO-ZnCr(2)O(4) catalysts for autothermal reforming of methanol
Liu, Na1,2; Yuan, Zhongshan1; Wang, Congwei3; Wang, Shudong1; Zhang, Chunxi1; Wang, Shujuan1
2008-06-01
发表期刊FUEL PROCESSING TECHNOLOGY
卷号89期号:6页码:574-581
摘要Autothermal reforming of methanol for hydrogen production was investigated over ZnO-ZnCr(2)O(4) supported on a series of metal oxides (Al(2)O(3), CeO(2), ZrO(2) and CeO(2)-ZrO(2))CeO(2)-ZrO(2) mixed oxides with Ce /Zr molar ratio of 4/1 was found to be the optimal support which showed significant effect on the catalytic activity and selectivity. The ZnO-ZnCr(2)O(4)/CeO(2)-ZrO(2) and ZnO-ZnCr(2)O(4) catalysts were characterized by XRD, TEM, H(2)-TPR and XPS. The results show that CeO(2)-ZrO(2) mixed oxides have significant effect on the catalytic performance and the supported catalyst shows more uniform temperature distribution in the catalyst bed which was mainly due to its reasonable redox properties. (C) 2007 Published by Elsevier B.V.
文章类型Article
关键词Hydrogen Production Methanol Autothermal Reforming Zno Ceo(2)-zro(2)
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.fuproc.2007.11.029
研究领域[WOS]Chemistry ; Energy & Fuels ; Engineering
关键词[WOS]ALCOHOL SYNTHESIS CATALYSTS ; FUEL-CELL APPLICATIONS ; HYDROGEN-PRODUCTION ; SURFACE CHARACTERIZATION ; CUO/CEO2 CATALYSTS ; REDOX BEHAVIOR ; ZN/CR SPINEL ; MIXED OXIDES ; PD/ZNO ; PERFORMANCE
收录类别SCI
语种英语
WOS类目Chemistry, Applied ; Energy & Fuels ; Engineering, Chemical
WOS记录号WOS:000256820600002
引用统计
被引频次:22[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10288
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China
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Liu, Na,Yuan, Zhongshan,Wang, Congwei,et al. The role of CeO(2)-ZrO(2) as support in the ZnO-ZnCr(2)O(4) catalysts for autothermal reforming of methanol[J]. FUEL PROCESSING TECHNOLOGY,2008,89(6):574-581.
APA Liu, Na,Yuan, Zhongshan,Wang, Congwei,Wang, Shudong,Zhang, Chunxi,&Wang, Shujuan.(2008).The role of CeO(2)-ZrO(2) as support in the ZnO-ZnCr(2)O(4) catalysts for autothermal reforming of methanol.FUEL PROCESSING TECHNOLOGY,89(6),574-581.
MLA Liu, Na,et al."The role of CeO(2)-ZrO(2) as support in the ZnO-ZnCr(2)O(4) catalysts for autothermal reforming of methanol".FUEL PROCESSING TECHNOLOGY 89.6(2008):574-581.
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