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Preparation of copper-iron bimodal pore catalyst and its performance for higher alcohols synthesis
Ding, Mingyue1; Liu, Jianguo1; Zhang, Qi1; Tsubaki, Noritatsu2; Wang, Tiejun1; Ma, Longlong1
2012-11-05
发表期刊CATALYSIS COMMUNICATIONS
卷号28页码:138-142
摘要

A multi-functional silica-silica bimodal pore catalyst support was prepared from silica sol and silica gel, which presented two kinds of main pores. Compared to the original silica gel, the obtained bimodal support had the enlarged surface area and decreased pore volume. This kind of bimodal pore support was applied firstly in higher alcohols synthesis, where both the copper and iron elements were supported as active sites. The bimodal pore catalyst exhibited favorite catalytic activity and high selectivity of C2+OH, due to the well dispersion of active metal sites and high diffusion efficiency of products inside the bimodal pore structures. Crown Copyright (C) 2012 Published by Elsevier B.V. All rights reserved.

文章类型Article
关键词Higher Alcohols Synthesis Bimodal Support Cu-fe Catalyst Syngas
WOS标题词Science & Technology ; Physical Sciences
DOI10.1016/j.catcom.2012.08.027
研究领域[WOS]Chemistry
关键词[WOS]FISCHER-TROPSCH SYNTHESIS ; CO HYDROGENATION ; MIXED ALCOHOLS ; SYNGAS
收录类别SCI
语种英语
WOS类目Chemistry, Physical
WOS记录号WOS:000311180800030
引用统计
被引频次:33[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10190
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Peoples R China
2.Toyama Univ, Sch Engn, Dept Appl Chem, Toyama 9308555, Japan
推荐引用方式
GB/T 7714
Ding, Mingyue,Liu, Jianguo,Zhang, Qi,et al. Preparation of copper-iron bimodal pore catalyst and its performance for higher alcohols synthesis[J]. CATALYSIS COMMUNICATIONS,2012,28:138-142.
APA Ding, Mingyue,Liu, Jianguo,Zhang, Qi,Tsubaki, Noritatsu,Wang, Tiejun,&Ma, Longlong.(2012).Preparation of copper-iron bimodal pore catalyst and its performance for higher alcohols synthesis.CATALYSIS COMMUNICATIONS,28,138-142.
MLA Ding, Mingyue,et al."Preparation of copper-iron bimodal pore catalyst and its performance for higher alcohols synthesis".CATALYSIS COMMUNICATIONS 28(2012):138-142.
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