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Directional synthesis of ethylbenzene through catalytic transformation of lignin
Fan, Minghui1; Jiang, Peiwen1; Bi, Peiyan1; Deng, Shumei1; Yan, Lifeng1; Zhai, Qi1; Wang, Tiejun2; Li, Quanxin1
2013-09-01
发表期刊BIORESOURCE TECHNOLOGY
卷号143页码:59-67
摘要Transformation of lignin to ethylbenzene can provide an important bulk raw material for the petrochemical industry. This work explored the production of ethylbenzene from lignin through the directional catalytic depolymerization of lignin into the aromatic monomers followed by the selective alkylation of the aromatic monomers. For the first step, the aromatics selectivity of benzene derived from the catalytic depolymerization of lignin reached about 90.2 C-mol% over the composite catalyst of Re-Y/HZSM-5 (25). For the alkylation of the aromatic monomers in the second step, the highest selectivity of ethylbenzene was about 72.3 C-mol% over the HZSM-5 (25) catalyst. The reaction pathway for the transformation of lignin to ethylbenzene was also addressed. Present transformation potentially provides a useful approach for the production of the basic petrochemical material and development of high-end chemicals utilizing lignin as the abundant natural aromatic resource. (C) 2013 Elsevier Ltd. All rights reserved.
文章类型Article
关键词Lignin Ethylbenzene Aromatic Monomer Depolymerization Alkylation
WOS标题词Science & Technology ; Life Sciences & Biomedicine ; Technology
DOI10.1016/j.biortech.2013.05.097
研究领域[WOS]Agriculture ; Biotechnology & Applied Microbiology ; Energy & Fuels
关键词[WOS]LIGHT OLEFINS ; BIO-OIL ; ALKYLATION ; BENZENE ; ZEOLITE ; CONVERSION ; DEPOLYMERIZATION ; ETHYLATION ; AROMATICS ; OXIDATION
收录类别SCI
语种英语
WOS类目Agricultural Engineering ; Biotechnology & Applied Microbiology ; Energy & Fuels
WOS记录号WOS:000323239800009
引用统计
被引频次:17[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10116
专题中国科学院广州能源研究所
作者单位1.Univ Sci & Technol China, Anhui Key Lab Biomass Clean Energy, Dept Chem Phys, Hefei 230026, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
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Fan, Minghui,Jiang, Peiwen,Bi, Peiyan,et al. Directional synthesis of ethylbenzene through catalytic transformation of lignin[J]. BIORESOURCE TECHNOLOGY,2013,143:59-67.
APA Fan, Minghui.,Jiang, Peiwen.,Bi, Peiyan.,Deng, Shumei.,Yan, Lifeng.,...&Li, Quanxin.(2013).Directional synthesis of ethylbenzene through catalytic transformation of lignin.BIORESOURCE TECHNOLOGY,143,59-67.
MLA Fan, Minghui,et al."Directional synthesis of ethylbenzene through catalytic transformation of lignin".BIORESOURCE TECHNOLOGY 143(2013):59-67.
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