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Hydrodeoxygenation of lignin-derived phenolic compounds to hydrocarbons over Ni/SiO2-ZrO2 catalysts
Zhang, Xinghua1,2; Zhang, Qi1; Wang, Tiejun1; Ma, Longlong1; Yu, Yuxiao1,2; Chen, Lungang1
2013-04-01
Source PublicationBIORESOURCE TECHNOLOGY
Volume134Pages:73-80
AbstractInexpensive non-sulfided Ni-based catalysts were evaluated for hydrodeoxygenation (HDO) using guaiacol as model compound. SiO2-ZrO2 (SZ), a complex oxide synthesized by precipitation method with different ratio of Si/Zr, was impregnated with Ni(NO3)(2)center dot 6H(2)O and calcined at 500 degrees C. Conversion rates and product distribution for guaiacol HDO at 200-340 degrees C were determined. Guaiacol conversion reached the maximum at 300 degrees C in the presence of Ni/SZ-3. When HDO reaction was carried out with real lignin-derived phenolic compounds under the optimal conditions determined for guaiacol, the total yield of hydrocarbons was 62.81%. These hydrocarbons were comprised of cyclohexane, alkyl-substituted cyclohexane and alkyl-substituted benzene. They have high octane number, would be the most desirable components for fungible liquid transportation fuel. (C) 2013 Elsevier Ltd. All rights reserved.
SubtypeArticle
KeywordSio2-zro2 Phenolic Compounds Hydrodeoxygenation (Hdo) Hydrocarbon
WOS HeadingsScience & Technology ; Life Sciences & Biomedicine ; Technology
DOI10.1016/j.biortech.2013.02.039
WOS Subject ExtendedAgriculture ; Biotechnology & Applied Microbiology ; Energy & Fuels
WOS KeywordNOBLE-METAL CATALYSTS ; BIO-OIL ; BIOMASS ; HYDROGENOLYSIS ; CONVERSION ; PYROLYSIS ; ZIRCONIA ; GUAIACOL ; SULFIDE ; ALKANES
Indexed BySCI
Language英语
WOS SubjectAgricultural Engineering ; Biotechnology & Applied Microbiology ; Energy & Fuels
WOS IDWOS:000328512800002
Citation statistics
Cited Times:136[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/10084
Collection中国科学院广州能源研究所
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Zhang, Xinghua,Zhang, Qi,Wang, Tiejun,et al. Hydrodeoxygenation of lignin-derived phenolic compounds to hydrocarbons over Ni/SiO2-ZrO2 catalysts[J]. BIORESOURCE TECHNOLOGY,2013,134:73-80.
APA Zhang, Xinghua,Zhang, Qi,Wang, Tiejun,Ma, Longlong,Yu, Yuxiao,&Chen, Lungang.(2013).Hydrodeoxygenation of lignin-derived phenolic compounds to hydrocarbons over Ni/SiO2-ZrO2 catalysts.BIORESOURCE TECHNOLOGY,134,73-80.
MLA Zhang, Xinghua,et al."Hydrodeoxygenation of lignin-derived phenolic compounds to hydrocarbons over Ni/SiO2-ZrO2 catalysts".BIORESOURCE TECHNOLOGY 134(2013):73-80.
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