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Synthesis gas production from biomass gasification using steam coupling with natural hematite as oxygen carrier
Huang, Zhen; He, Fang; Zheng, Anqing; Zhao, Kun; Chang, Sheng; Zhao, Zengli; Li, Haibin
2013-05-01
发表期刊ENERGY
卷号53页码:244-251
摘要Biomass gasification using lattice oxygen (BGLO) of natural hematite coupling with steam was conducted in a fluidized bed reactor. The presence of hematite particles evidently facilitated to biomass gasification. Comparing with biomass steam gasification (BSG), carbon conversion and gas yield increased by 7.47% and 11.02%, respectively, and tar content lowered by 51.53%, in BGLO with an S/B of 0.85 at 800 degrees C. In this case, 62.30% of the lattice oxygen in the hematite particles was consumed in the biomass gasification. The reaction temperature, steam-to-biomass ratio (S/B) and reaction time on the performance of hematite particles were extensively investigated, in terms of gas distribution, heating value, yield and carbon conversion. With the reaction temperature increasing from 750 to 850 degrees C, the gas yield increased from1.12 to 1.53Nm(3)/kg, and carbon conversion increased from 77.21% to 95.49%. An optimal S/B ratio of 0.85 was obtained in order to maximize the carbon conversion and gas yield of BGLO. At this ratio, the gas yield reached 1.41Nm(3)/kg with carbon conversion of 92.98%. The gas concentration was gradually close to that of BSG at the end stage of BGLO due to the active lattice oxygen was depleted with the proceeding of reactions. (C) 2013 Elsevier Ltd. All rights reserved.
文章类型Article
关键词Biomass Gasification Lattice Oxygen Oxygen Carrier Natural Hematite Fluidize Bed Reactor
WOS标题词Science & Technology ; Physical Sciences ; Technology
DOI10.1016/j.energy.2013.02.068
研究领域[WOS]Thermodynamics ; Energy & Fuels
关键词[WOS]CHEMICAL-LOOPING COMBUSTION ; HYDROGEN-RICH GAS ; FLUIDIZED-BED ; SOLID FUELS ; CO2 CAPTURE ; AIR ; GENERATION ; CATALYSTS ; OLIVINE ; CYCLE
收录类别SCI
语种英语
WOS类目Thermodynamics ; Energy & Fuels
WOS记录号WOS:000318455600027
引用统计
被引频次:86[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10065
专题中国科学院广州能源研究所
作者单位Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate CAS, Guangzhou 510640, Guangdong, Peoples R China
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Huang, Zhen,He, Fang,Zheng, Anqing,et al. Synthesis gas production from biomass gasification using steam coupling with natural hematite as oxygen carrier[J]. ENERGY,2013,53:244-251.
APA Huang, Zhen.,He, Fang.,Zheng, Anqing.,Zhao, Kun.,Chang, Sheng.,...&Li, Haibin.(2013).Synthesis gas production from biomass gasification using steam coupling with natural hematite as oxygen carrier.ENERGY,53,244-251.
MLA Huang, Zhen,et al."Synthesis gas production from biomass gasification using steam coupling with natural hematite as oxygen carrier".ENERGY 53(2013):244-251.
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