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Phase Equilibrium Data of Tetrabutylphosphonium Bromide Plus Carbon Dioxide or Nitrogen Semiclathrate Hydrates
Shi, Ling-Li1,2; Liang, De-Qing1; Li, Dong-Liang1
2013-07-01
Source PublicationJOURNAL OF CHEMICAL AND ENGINEERING DATA
Volume58Issue:7Pages:2125-2130
AbstractIn this paper, phase equilibrium data of tetrabutylphosphonium bromide (TBPB) + CO2, + N-2 semiclathrate hydrates were measured by employing an isochoric pressure-search method. The experimental temperature, pressure, and mass fraction of TBPB ranged from (282.2 to 292.0) K, from (1.32 to 16.86) MPa, and from (0.050 to 0.600), respectively. The results demonstrated that at a given pressure, the temperature required to form mixed TBPB + CO2, + N-2 hydrates was significantly higher than that required for forming pure Co-2 or N-2 hydrates. In addition, the application of TBPB at 0.371 mass fraction, responding to TBPB center dot 32H(2)O, showed the strongest stabilization effect.
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1021/je400452f
WOS Subject ExtendedChemistry ; Engineering
WOS KeywordSEMI-CLATHRATE HYDRATE ; TETRABUTYL AMMONIUM-NITRATE ; AQUEOUS-SOLUTION SYSTEMS ; HYDROGEN STORAGE ; THERMODYNAMIC STABILITY ; DISSOCIATION ENTHALPIES ; PHOSPHONIUM BROMIDE ; COLD-STORAGE ; CO2 ; GAS
Indexed BySCI
Language英语
WOS SubjectChemistry, Multidisciplinary ; Engineering, Chemical
WOS IDWOS:000321883700028
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Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/10052
Collection中国科学院广州能源研究所
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Shi, Ling-Li,Liang, De-Qing,Li, Dong-Liang. Phase Equilibrium Data of Tetrabutylphosphonium Bromide Plus Carbon Dioxide or Nitrogen Semiclathrate Hydrates[J]. JOURNAL OF CHEMICAL AND ENGINEERING DATA,2013,58(7):2125-2130.
APA Shi, Ling-Li,Liang, De-Qing,&Li, Dong-Liang.(2013).Phase Equilibrium Data of Tetrabutylphosphonium Bromide Plus Carbon Dioxide or Nitrogen Semiclathrate Hydrates.JOURNAL OF CHEMICAL AND ENGINEERING DATA,58(7),2125-2130.
MLA Shi, Ling-Li,et al."Phase Equilibrium Data of Tetrabutylphosphonium Bromide Plus Carbon Dioxide or Nitrogen Semiclathrate Hydrates".JOURNAL OF CHEMICAL AND ENGINEERING DATA 58.7(2013):2125-2130.
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