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Investigation on the Aqueous-phase Hydrogenation of Bio-oil for Saturated Alcohols Production over Ni-B Amorphous Catalysts
Yu Yu-Xiao1,2; Zhang Xing-Hua1,2; Wang Tie-Jun1; Xu Ying1; Ma Long-Long1; Zhang Qi1; Zhang Li-Min3
2013-09-10
发表期刊CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE
卷号34期号:9页码:2178-2183
摘要Ni-B amorphous catalysts were prepared by chemical reduction of nickel chloride with potassium borohydride aqueous solution and characterized by X-ray diffraction(XRD), Brunauer-Emmett-Tetter(BET), scanning electron microscopy (SEM), transmission electron microscopy (TEM), inductively coupled plasma (ICP) techniques. The catalytic performances of model compounds and bio-oil to produce saturated alcohols were evaluated in a semi-batch reactor. The results showed that the conversion of model compounds(acetone, furfural and phenol) and the selectivity of saturated alcohols reached 99.99% and 90.00% at 110 degrees C, 4.0 MPa(initial pressure). Under the conditions of 150 degrees C and 4.0 MPa, the yield of saturated alcohols reached 47.54%. High temperature of above 150 degrees C resulted in the transformation of amorphous phase to form crystal, which was attributed to the low catalytic activity. This work provides a new alternative for the production of saturated alcohols from bio-oil.
文章类型Article
关键词Bio-oil Ni-b Catalyst Aqueous-phase Reforming Saturated Alcohol
WOS标题词Science & Technology ; Physical Sciences
DOI10.7503/cjcu20130258
研究领域[WOS]Chemistry
关键词[WOS]ALLOY CATALYST ; PYROLYSIS OIL ; HYDRODEOXYGENATION ; BIOMASS ; HYDROTREATMENT ; PHENOL ; LA
收录类别SCI
语种英语
WOS类目Chemistry, Multidisciplinary
WOS记录号WOS:000328926400026
引用统计
被引频次:4[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10047
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Changsha Univ Sci & Technol, Coll Chem & Biol Engn, Changsha 410004, Hunan, Peoples R China
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Yu Yu-Xiao,Zhang Xing-Hua,Wang Tie-Jun,et al. Investigation on the Aqueous-phase Hydrogenation of Bio-oil for Saturated Alcohols Production over Ni-B Amorphous Catalysts[J]. CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,2013,34(9):2178-2183.
APA Yu Yu-Xiao.,Zhang Xing-Hua.,Wang Tie-Jun.,Xu Ying.,Ma Long-Long.,...&Zhang Li-Min.(2013).Investigation on the Aqueous-phase Hydrogenation of Bio-oil for Saturated Alcohols Production over Ni-B Amorphous Catalysts.CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,34(9),2178-2183.
MLA Yu Yu-Xiao,et al."Investigation on the Aqueous-phase Hydrogenation of Bio-oil for Saturated Alcohols Production over Ni-B Amorphous Catalysts".CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE 34.9(2013):2178-2183.
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