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Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts
Zhang, Xinghua1,2; Wang, Tiejun1; Ma, Longlong1; Zhang, Qi1; Huang, Xiaoming1,2; Yu, Yuxiao1,2
2013-12-01
发表期刊APPLIED ENERGY
卷号112页码:533-538
摘要The main products of lignin degradation are phenolic compounds. It is meaningful to study the processes by which cyclohexane is produced from phenolic compounds via hydrodeoxygenation (HDO), because it could be used as fuel additives, chemical feedstock and solvent. In this work, support material ZrO2-SiO2 mixed oxides with different Si/Zr ratio were synthesized, and a series of Ni/SiO2-ZrO2 catalysts with different Ni loading were prepared by impregnation method. The exploration of HDO process was carried out using phenol and guaiacol as model compounds. Effects of Si/Zr ratio, Ni loading and reaction temperature on conversion of phenol and guaiacol as well as distribution of HDO products were systematically investigated. The results showed that almost all of phenol and guaiacol could be effectively converted into O-free products. And the selectivity of cyclohexane was in excess of 90%. (C) 2013 Elsevier Ltd. All rights reserved.
文章类型Article
关键词Lignin Phenolic Compounds Ni/zro2-sio2 Cyclohexane Hydrodeoxygenation (Hdo)
WOS标题词Science & Technology ; Technology
DOI10.1016/j.apenergy.2013.04.077
研究领域[WOS]Energy & Fuels ; Engineering
关键词[WOS]ETHANOL-PRODUCTION ; HYDRODEOXYGENATION ; CONVERSION ; ACID
收录类别SCI ; ISTP
语种英语
WOS类目Energy & Fuels ; Engineering, Chemical
WOS记录号WOS:000329377800056
引用统计
被引频次:90[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.giec.ac.cn/handle/344007/10035
专题中国科学院广州能源研究所
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Peoples R China
2.Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China
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Zhang, Xinghua,Wang, Tiejun,Ma, Longlong,et al. Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts[J]. APPLIED ENERGY,2013,112:533-538.
APA Zhang, Xinghua,Wang, Tiejun,Ma, Longlong,Zhang, Qi,Huang, Xiaoming,&Yu, Yuxiao.(2013).Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts.APPLIED ENERGY,112,533-538.
MLA Zhang, Xinghua,et al."Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts".APPLIED ENERGY 112(2013):533-538.
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