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Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts
Zhang, Xinghua1,2; Wang, Tiejun1; Ma, Longlong1; Zhang, Qi1; Huang, Xiaoming1,2; Yu, Yuxiao1,2
2013-12-01
Source PublicationAPPLIED ENERGY
Volume112Pages:533-538
AbstractThe main products of lignin degradation are phenolic compounds. It is meaningful to study the processes by which cyclohexane is produced from phenolic compounds via hydrodeoxygenation (HDO), because it could be used as fuel additives, chemical feedstock and solvent. In this work, support material ZrO2-SiO2 mixed oxides with different Si/Zr ratio were synthesized, and a series of Ni/SiO2-ZrO2 catalysts with different Ni loading were prepared by impregnation method. The exploration of HDO process was carried out using phenol and guaiacol as model compounds. Effects of Si/Zr ratio, Ni loading and reaction temperature on conversion of phenol and guaiacol as well as distribution of HDO products were systematically investigated. The results showed that almost all of phenol and guaiacol could be effectively converted into O-free products. And the selectivity of cyclohexane was in excess of 90%. (C) 2013 Elsevier Ltd. All rights reserved.
SubtypeArticle
KeywordLignin Phenolic Compounds Ni/zro2-sio2 Cyclohexane Hydrodeoxygenation (Hdo)
WOS HeadingsScience & Technology ; Technology
DOI10.1016/j.apenergy.2013.04.077
WOS Subject ExtendedEnergy & Fuels ; Engineering
WOS KeywordETHANOL-PRODUCTION ; HYDRODEOXYGENATION ; CONVERSION ; ACID
Indexed BySCI ; ISTP
Language英语
WOS SubjectEnergy & Fuels ; Engineering, Chemical
WOS IDWOS:000329377800056
Citation statistics
Cited Times:53[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/10035
Collection中国科学院广州能源研究所
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Peoples R China
2.Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Xinghua,Wang, Tiejun,Ma, Longlong,et al. Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts[J]. APPLIED ENERGY,2013,112:533-538.
APA Zhang, Xinghua,Wang, Tiejun,Ma, Longlong,Zhang, Qi,Huang, Xiaoming,&Yu, Yuxiao.(2013).Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts.APPLIED ENERGY,112,533-538.
MLA Zhang, Xinghua,et al."Production of cyclohexane from lignin degradation compounds over Ni/ZrO2-SiO2 catalysts".APPLIED ENERGY 112(2013):533-538.
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